A single source femtosecond-millisecond broadband spectrometer

E. C. Carroll; M. P. Hill; D. MadsenK. R. MalleyD. S. Larsen

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A single source femtosecond-millisecond broadband spectrometer

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Time-resolved measurement of population dynamics extending over femtosecond to millisecond time scales typically requires a combination of transient absorption techniques involving different laser systems and detection schemes. The spectrometer design presented here facilitates transient absorption measurements over 12 decades with a single ultrafast laser system by picking pump and probe pulses independently from the laser oscillator pulse train. Unamplified pulses seed a photonic crystal fiber to a supercontinuum probe source for spectrally resolved measurements. The utility of the system is demonstrated by measuring triplet state dynamics following photoexcitation of vitamin B_(6) in aqueous solution.

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《Review of Scientific Instruments》 |2009年第2期|026102-1-026102-3-0|共3页
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E. C. Carroll; M. P. Hill; D. MadsenK. R. MalleyD. S. Larsen;
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Department of Chemistry, University of California, Davis, One Shields Avenue, Davis, California 95616, USA;

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正文语种英语
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A single source femtosecond-millisecond broadband spectrometer

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