Highly selective co-production of nitrocyclohexane and adipic acid from vapor phase catalytic nitration-oxidation of cyclohexane with NO2

Kuiyi You; Jian Jian; Haijun Xiao

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Highly selective co-production of nitrocyclohexane and adipic acid from vapor phase catalytic nitration-oxidation of cyclohexane with NO2

机译：气相催化硝化氧化环己烷与NO2的高选择性联产硝基环己烷和己二酸

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摘要

A simple and efficient approach for highly selectivity co-production of nitrocyclohexane and adipic acid from vapor phase nitration-oxidation of cyclohexane with NO2 at atmospheric pressure has been successfully developed in this work. This finding provides a novel strategy for co-production of nitroalkanes and dicarboxylic acids from vapor phase nitration-oxidation of low-carbon cycloalkanes. This method may be very significant to establish such a synthesis process for aliphatic nitro-compounds and dicarboxylic acids in organic fields.

机译：在这项工作中，已经成功开发了一种简单高效的方法，用于在大气压力下由环己烷与NO2进行气相硝化-氧化，高选择性地联产硝基环己烷和己二酸。这一发现为低碳环烷烃的气相硝化-氧化共生产硝基烷和二羧酸提供了一种新的策略。该方法对于建立有机领域中的脂肪族硝基化合物和二羧酸的合成方法可能非常重要。

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来源
《Catalysis Communications》 |2012年第null期|共5页
作者
Kuiyi You; Jian Jian; Haijun Xiao;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
关键词
Catalytic nitration-oxidation; Vapor phase; Co-production; Nitrocyclohexane; Adipic acid;

机译：催化硝化-氧化;气相;联产;硝基环己烷;己二酸;

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1. Highly selective co-production of nitrocyclohexane and adipic acid from vapor phase catalytic nitration-oxidation of cyclohexane with NO2 [J] . Kuiyi You, Jian Jian, Haijun Xiao Catalysis Communications . 2012,第Null期

机译：气相催化硝化氧化环己烷与NO2的高选择性联产硝基环己烷和己二酸
2. A simple and efficient approach for highly selective preparation of nitrocyclohexane from cyclohexane with tert-butyl nitrite catalyzed by N-hydroxyphthalimide [J] . Liu Shuilin, You Kuiyi, Jian Jian, Research on Chemical Intermediates . 2016,第3期

机译：N-羟基邻苯二甲酰亚胺催化的亚硝酸叔丁酯从环己烷中高选择性制备硝基环己烷的简单有效方法
3. Vapor Phase Selective Catalytic Oxidation of Cyclohexane over 13X Supported Metal Oxides in the Presence of Ozone [J] . Gopi T., Swetha G., Shekar S. Chandra, Ozone: Science & Engineering: The Journal of the International Ozone Association . 2016,第6期

机译：臭氧存在下13X负载金属氧化物上环己烷的气相选择性催化氧化
4. Highly efficient Nano-catalysts Using Activated Carbon as a Support for One-step Oxidation of Cyclohexane to Adipic Acid [C] . H.Dai, M.Zhu, W.Li, Annual conference of the Chinese Society of Micro-Nano technology;International conference of the Chinese Society of Micro-Nano technology;International workshop on innovation and commercialization of Micro & Nanotechnology . 2012

机译：使用活性炭作为载体，将环己烷一步氧化为己二酸的高效纳米催化剂
5. Selective dehydration of polyols over solid acids and metal-acid bifunctional catalysts: Towards a catalytic toolbox for rational catalyst design. [D] . Nolan, Michael R. 2014

机译：在固体酸和金属酸双功能催化剂上进行多元醇的选择性脱水：成为合理设计催化剂的催化工具箱。
6. Facile preparation of highly-dispersed cobalt-silicon mixed oxide nanosphere and its catalytic application in cyclohexane selective oxidation [O] . Qiaohong Zhang, Chen Chen, Min Wang, 2011

机译：高分散钴硅混合氧化物纳米球的简便制备及其在环己烷选择性氧化中的催化应用
7. Vapor phase Beckmann rearrangement over highly silicious ZSM-5. II. Special articles on zeolite chemistry and technology. Relations between the zeolitic properties of ZSM-5 and its catalytic activities for a vapor-phase Beckmann rearrangement. [O] . Hiroshi SATO, Kenichi HIROSE, Masaru KITAMURA 1989

机译：蒸汽相位贝克曼重新排列高度硅基-5。 II。关于沸石化学和技术的特殊文章。 ZSM-5沸石特性与蒸汽相贝克曼重排的催化活性的关系。

Highly selective co-production of nitrocyclohexane and adipic acid from vapor phase catalytic nitration-oxidation of cyclohexane with NO2

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