Chemodosimeter for fluoride ions based on F--triggered Si-O cleavage followed by the deprotonation/autoxidation of secondary nitrile C-H group

Li Baiyun; Zhang Chuanxiu; Liu Chuanxiang; Chen Jinju; Wang Xinyu; Liu Zhenjiang; Yi Fengping

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Chemodosimeter for fluoride ions based on F--triggered Si-O cleavage followed by the deprotonation/autoxidation of secondary nitrile C-H group

机译：基于F-触发的Si-O裂解然后继发腈C-H基团去质子/自动氧化的氟离子化学计量仪

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摘要

A completely new strategy for a chemodosimeter for fluoride based on F--triggered Si-O bond cleavage, followed by the deprotonation/autoxidation of secondary nitrile C-H group was developed for the first time. The chemodosimeter exhibited high selectivity and sensitivity, dramatic color "turn-on", and fluorescence "turn-off" for the detection for fluoride.

机译：首次开发了一种基于F触发的Si-O键裂解的氟化物化学计量仪的全新策略，随后是次腈C-H基团的去质子化/自氧化。化学光度计显示出高的选择性和灵敏度，显着的颜色“打开”和荧光“关闭”，用于检测氟化物。

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《RSC Advances》 |2014年第86期|共4页
作者
Li Baiyun; Zhang Chuanxiu; Liu Chuanxiang; Chen Jinju; Wang Xinyu; Liu Zhenjiang; Yi Fengping;
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正文语种 eng
中图分类化学;
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1. Chemodosimeter for fluoride ions based on F--triggered Si-O cleavage followed by the deprotonation/autoxidation of secondary nitrile C-H group [J] . Li Baiyun, Zhang Chuanxiu, Liu Chuanxiang, RSC Advances . 2014,第86期

机译：基于F-触发的Si-O裂解然后继发腈C-H基团去质子/自动氧化的氟离子化学计量仪
2. Chromogenic and fluorescent "turn-on' chemodosimeter for fluoride based on a F--triggered cascade reaction [J] . Li Baiyun, Zhang Chuanxiu, Wang Yu, Luminescence: The journal of biological and chemical luminescence . 2015,第5期

机译：基于F触发的级联反应的氟化物的发色和荧光“开启”化学计量仪
3. A near-infrared fluorescence chemodosimeter for fluoride via specific Si-O cleavage [J] . Jian Cao, Chunchang Zhao, Weihong Zhu Tetrahedron letters: The International Journal for the Rapid Publication of Preliminary Communications in Organic Chemistry . 2012,第16期

机译：通过特定的Si-O裂解来检测氟化物的近红外荧光化学计量仪
4. A Ruthenium-Catalyzed Reaction of Aromatic Ketones with Organoboronic Acid Esters:A New Method for C-C Bond Formation via C-H Bonds Cleavage [C] . Fumitoshi Kakiuchi, Shintaro Kan, Kimitaka Igi, Symposium on Organometallic Chemistry . 2003

机译：芳香酮与有机硼酸酯的芳香酮催化反应：通过C-H键切割的C-C键形成新方法
5. Part A. Diastereoselective synthesis of protected secondary amines via reduction /alkylation or deprotonation /alkylation of N-diphenylphosphinylimines. Part B. Synthesis of secondary amines via 1,2-addition of organometallic reagents to N-diphenylphosphinylimines and subsequent alkylation [D] . Shin, Hyunshun 2001

机译：A部分：通过N-二苯基膦亚胺的还原/烷基化或去质子化/烷基化的非对映选择性合成保护的仲胺。 B部分：通过将有机金属试剂1,2-加成到N-二苯基膦亚胺和随后的烷基化反应来合成仲胺
6. Meta-Selective C-H Functionalization using a Nitrile based Directing Group and Cleavable Si-Tether [O] . Sunggi Lee, Hyelee Lee, Kian L. Tan -1

机译：使用基于腈的导向基团和可裂解的硅系链进行亚选择性C-H功能化
7. Incorporation of the fluoride induced Si-O bond cleavage and functionalized gold nanoparticle aggregation into one colorimetric probe for highly specific and sensitive detection of fluoride [O] . Sun Jie-Fang, Liu Rui, Zhang Zhong-Mian, 2014

机译：将氟化物诱导的Si-O键断裂和功能化的金纳米粒子聚集体结合到一个比色探针中，以高度特异性和灵敏地检测氟化物
8. Redox Catalysis Involving Substrate Photooxidation with Catalyst Regeneration bySubstrate Reduction. Simultaneous Oxidative C-H Bond Cleavage and Reductive C-S Bond Cleavage in Thioethers Catalyzed by W10O324- [R] . Chambers, R. C., Hill, C. L. 1990

机译：氧化还原催化与底物光氧化反应的催化剂再生通过底物还原。 W10O324催化的硫醚同时氧化C-H键断裂和还原C-s键断裂

Chemodosimeter for fluoride ions based on F--triggered Si-O cleavage followed by the deprotonation/autoxidation of secondary nitrile C-H group

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