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Single-shot imaging of ground-state hydrogen atoms with a nonlinear laser spectroscopic technique

机译:利用非线性激光光谱技术对基态氢原子进行单次成像

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摘要

We report on a novel nonlinear laser spectroscopic technique for single-shot imaging of ground-state hydrogenatoms in harsh environments. H atoms from the ground state were first pumped to the 2s state via a two-photon excitation with a 243 nm laser beam, and the population of the 2s state was further probed through the 2s-4p transition with conventional polarization spectroscopy at 486 nm. A single Nd:YAG-pumped optical parametric oscillator laser system was enough to provide both laser beams. Single-shot visualization of native H atoms in an atmospheric pressure premixed H_(2)/O_(2) flame is demonstrated.
机译:我们报告了一种新颖的非线性激光光谱技术,用于在恶劣环境下对基态氢原子进行单次成像。首先将来自基态的H原子通过243 nm激光束通过双光子激发泵浦到2s状态,然后使用486 nm的常规偏振光谱通过2s-4p跃迁进一步探测2s状态的种群。单个Nd:YAG泵浦光参量振荡器激光系统足以提供两个激光束。演示了大气压预混合H_(2)/ O_(2)火焰中天然H原子的单次可视化。

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