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FUNCTIONALIZATION OF ORGANIC MOLECULES USING METAL-ORGANIC FRAMEWORKS (MOFS) AS CATALYSTS
FUNCTIONALIZATION OF ORGANIC MOLECULES USING METAL-ORGANIC FRAMEWORKS (MOFS) AS CATALYSTS
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机译:以金属有机骨架(MOFS)为催化剂的有机分子功能化
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摘要
1. A method of replacing at least one atom of an organic molecule with another atom or group of atoms, by contacting the molecule with Organometallic strukturoy.2. A method according to Claim. 1, wherein the organic molecule is a uglevodorod.3. A method according to Claim. 1, wherein the hydrogen in the organic molecule is replaced by an oxygen-containing functional gruppoy.4. A method according to Claim. 1, wherein the method is carried out in the presence CO.5. A method according to Claim. 1, wherein the method is carried out in the presence okislitelya.6. A method according to Claim. 1, wherein the organic molecule is an alkane, which is converted to a carboxylic kislotu.7. A method according to Claim. 1, wherein the organometallic structure comprises a metal or metal ion including alkali metal, alkaline earth metal, transition metal, lanthanide, actinide, metalloid, or post-transition metall.8. . A method according to claim 7, wherein the organometallic structure comprises a metal or metal ion selected from the group consisting of: Li, Na, K, Rb, Cs, Be, Mg, Ca, Sr, Ba, Sc, Sc, Sc, Y , Y, Y, Ti, Ti, Ti, Zr, Zr, Zr, Hf, Hf, V, V, V, V, Nb, Nb, Nb, Nb, Ta, Ta, Ta, Ta, Cr, Cr, Cr , Cr, Cr, Cr, Cr, Mo, Mo, Mo, Mo, Mo, Mo, Mo, W, W, W, W, W, W, W, Mn, Mn, Mn, Mn, Mn, Mn, Mn , Re, Re, Re, Re, Re, Re, Re, Re, Fe, Fe, Fe, Fe, Fe, Fe, Ru, Ru, Ru, Ru, Ru, Ru, Os, Os, Os, Os, Os , Os, Os, Os, Os, Co, Co, Co, Co, Co, Rh, Rh, Rh, Rh, Rh, Rh, Ir, Ir, Ir, Ir, Ir, Ir, Ir, Ni, Ni, Ni , Ni, Pd, Pd, Pd, Pd, Pd, Pt, Pt. Pt, Pt, Pt, Pt, Cu, Cu, Cu, Cu, Ag, Ag, Ag, Au, Au, Au, Au, Au, Zn, Zn, Zn, Cd, Cd, Hg, Hg, Hg, B, B, B, Al, Al, Al, Ga, Ga, Ga, In, In, In, Tl, Tl, Si, Si, Si, Si, Ge, Ge, Ge, Ge, Ge, Sn, Sn, Pb, Pb, As, As, As, As, Sb, Sb, Bi, Bi, Te, Te, Te, Te, La, La, Ce, Ce, Ce, Pr, Pr, Pr, Nd, Nd, Sm, Sm, eu, eu, Gd, Gd, Gd, Tb, Tb, Tb, Tb, Dy, Dy, Ho, Er, Tm, Tm, Tm, Yb, Ybi Lu.9. A method according to Claim. 1, wherein the organometallic structure comprises a metal or metal ion having a molecular geometry selected from the group consisting of planar trigonal, tetrahedral, square planar, trigonal
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