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THE TWO-ELECTRON RESPONSE IN LASER DRIVEN HELIUM

机译:激光驱动氦气中的两种电子响应

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The four main goals of our full-dimensionality integration of the Time-Dependent Schroedinger Equation (TDSE) have been to: 1. Enable the calculation of intense-field (two-electron) phenomena that no low-dimensionality or ad hoc theory can adequately model. 2. Support the design of simplified theoretical models of multi-electron, atom-laser interactions and assess their ranges of validity. 3. Support, interpret and guide laboratory experiment. 4. Provide a stepping stone towards a full-dimensional treatment of the 3-body and 4-body problems presented by laser-driven H_2~+ and H_2 which are of fundamental importance to femto-second Chemistry In this paper, attention is focussed on points 1 and 3 above. A description of the method and associated computer algorithms is given in section 2. Section 3 concentrates on recent results obtained at a laser wavelength of 390 nm which take the form of ratios of double- to single-ionization yields. A direct comparison with experimental work is presented. Section 4 gives details of an investigation into ionization dynamics at a laser wavelength of 20.6 nm. Momentum distributions for doubly-ionizing wavepackets are given and preliminary results on two-electron above threshold ionization are reported.
机译:我们对时变Schroedinger方程(TDSE)进行全维积分的四个主要目标是:1.启用对强场(双电子)现象的计算,这是低维或即席理论无法充分实现的模型。 2.支持设计多电子,原子-激光相互作用的简化理论模型,并评估其有效性范围。 3.支持,解释和指导实验室实验。 4.为全面解决由激光驱动的H_2〜+和H_2引起的3体和4体问题提供了垫脚石,这对飞秒化学至关重要。本文将重点放在以上的第1点和第3点。在第2节中介绍了该方法和相关的计算机算法。第3节重点介绍了在390 nm激光波长下获得的最新结果,该结果采用双电离与单电离产率的比值形式。提出了与实验工作的直接比较。第4节详细介绍了在20.6 nm激光波长下的电离动力学研究。给出了双电离波包的动量分布,并报告了高于阈值电离的两个电子的初步结果。

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