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Ultrafast energy flow in hybrid plasmonic materials

机译:混合等离子体材料中的超快能量流

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Nanoscale materials absorb, propagate, and dissipate energy very differently than their bulk counterparts. Furthermore, hybrid nanostructures consisting of molecular and plasmonic materials with strongly coupled electronic states can produce new optical states and decay pathways that provide additional handles with which to externally control energy flow in complex nanostructured systems. In this talk, we discuss our recent studies of electromagnetic coupling and associated temporal dynamics of molecular excitations with plasmonic resonances supported by either localized or extended planar geometries. Recent experimental results and theoretical analysis for observing and controlling coherences between molecular excitations and plasmonic polarizations are shown. Advances will explore new directions in ultrafast manipulation of energy dissipation processes in hybrid plasmonic structures, as well as ultrafast addressing and switching in plasmonics-based circuit architectures. Also discussed are recent synthetic advances in the creation of hybrid materials. Ultimately, these studies may impact a range of next-generation optical materials and devices, of relevance to new energy conversion materials, nanoscale photocatalysis, or plasmon-enhanced sensors.
机译:纳米材料与大体积材料相比,吸收,传播和耗散能量的方式非常不同。此外,由具有强耦合电子状态的分子和等离激元材料组成的杂化纳米结构可以产生新的光学状态和衰减路径,从而提供额外的控制柄,从而可以从外部控制复杂纳米结构系统中的能量流。在本次演讲中,我们讨论了我们最近对具有局部或扩展平面几何形状的等离子共振的分子激发的电磁耦合和相关时间动力学的研究。显示了用于观察和控制分子激发和等离子体极化之间相干性的最新实验结果和理论分析。先进技术将探索混合等离子体结构中能量耗散过程的超快速处理以及基于等离子体的电路架构中超快速寻址和切换的新方向。还讨论了混合材料创建中的最新合成进展。最终,这些研究可能会影响与新能量转换材料,纳米级光催化或等离激元增强传感器相关的下一代光学材料和设备。

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