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Why does surface ozone peak before a typhoon landing in southeast China?

机译:为什么在台风登陆中国东南之前,地表臭氧达到峰值?

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A high O3 episode with the large increases in surface ozone by21–42 ppbv and the nocturnal surface O3 levels exceeding 70 ppbv wasobserved in the region between Xiamen and Quanzhou over the southeasterncoast of China during 12–14 June 2014, before the Typhoon Hagibis landing.Variations in the surface O3, NO2, CO and meteorology during theTyphoon Hagibis event clearly suggest a substantial impact of the peripheraldowndrafts in the large-scale typhoon circulation on such an O3 episodeexcluding the contributions of photochemical production and the horizontaltransport. The influence of vertical O3 transport from the uppertroposphere and lower stratosphere (UTLS) region on high surface O3levels is further confirmed by a negative correlation between surface O3and CO concentrations as well as dry surface air observed during the O3episode. This study provides observational evidence of typhoon-drivenintrusion of O3 from the UTLS region to surface air, revealing asignificant effect of such a process of stratosphere–troposphere exchange(STE) of O3 on tropospheric O3 and ambient air quality.
机译:在厦门和泉州之间的区域内,观测到了一个高O 3 事件,表面臭氧增加了21-42 ppbv,夜间地面O 3 水平超过70 ppbv。 2014年6月12日至14日,在台风哈吉比登陆前的中国东南沿海。台风哈吉比事件期间地面O 3 ,NO 2 ,CO和气象的变化明确表明大规模台风环流的外围下降气流对这种O 3 事件的影响很大,但不包括光化学产生和水平输送的贡献。表面O 之间的负相关性进一步证实了来自高空对流层和低平流层(UTLS)区域的垂直O 3 传输对高表面O 3 水平的影响。 O 3 事件中观测到的3 和CO浓度以及表面干燥的空气。这项研究提供了台风驱动的O 3 从UTLS区域侵入地面空气的观测证据,揭示了O 3 3 和周围空气质量。

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