首页> 外文期刊>Environmental toxicology and chemistry >RELATIONSHIP BETWEEN POLYCHLORINATED DIBENZO-p-DIOXIN, POLYCHLORINATED DIBENZOFURAN, AND DIOXIN-LIKE POLYCHLORINATED BIPHENYL CONCENTRATIONS IN VEGETATION AND SOIL ON RESIDENTIAL PROPERTIES
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RELATIONSHIP BETWEEN POLYCHLORINATED DIBENZO-p-DIOXIN, POLYCHLORINATED DIBENZOFURAN, AND DIOXIN-LIKE POLYCHLORINATED BIPHENYL CONCENTRATIONS IN VEGETATION AND SOIL ON RESIDENTIAL PROPERTIES

机译:植被和土壤中多氯联苯对二恶英,多氯联苯呋喃和类似二恶英的多氯联苯浓度在土壤和土壤中的关系

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摘要

The University of Michigan Dioxin Exposure Study was undertaken to address concerns that the industrial discharge of dioxin-like compounds in the Midland, Michigan, USA area had resulted in the contamination of soil and vegetation in the Tittabawassee River floodplain and downwind of the incinerator in the City of Midland. The study included the analysis of 597 vegetation samples, predominantly grass and weeds, from residential properties selected through a multistage probabilistic sample design in the Midland area, and in Jackson and Calhoun Counties (Michigan), as a background comparison, for 29 polychlorinated dibenzo-p-dioxins (PCDDs), polychlorinated dibenzofurans (PCDFs), and polychlorinated biphenyls (PCBs). The mean toxic equivalent (TEQ) of the house perimeter vegetation samples ranged from 4.2 to 377 pg/g. The ratio of TEQs (vegetation to soil) was about 0.3, with a maximum of 3.5. Based on a calculation of the similarity of the congener patterns between the soil and the vegetation, it appeared that the source of the contamination on the vegetation was the surrounding soil. This conclusion was supported by linear regression analysis, which showed that the largest contributor to the R~2 for the outcome variable of log_(10) of the vegetation concentration was log_(10) of the surrounding soil concentration. Models of vegetation contamination usually focus on atmospheric deposition and partitioning. The results obtained here suggest that the deposition of soil particles onto vegetation is a significant route of contamination for residential herbage. Thus, the inclusion of deposition of soil particles onto vegetation is critical to the accurate modeling of contamination residential herbage in communities impacted by historic industrial discharges of persistent organic compounds.
机译:密歇根大学对二恶英的暴露进行了研究,以解决人们担心的问题,即美国密歇根州米德兰地区的二恶英类化合物的工业排放已导致蒂塔巴瓦湖河洪泛区的土壤和植被受到污染,以及该地区焚化炉的顺风。米德兰市。该研究包括分析米德兰地区以及密歇根州杰克逊县和卡尔霍恩县(密歇根州)通过多阶段概率抽样设计选择的住宅物业中的597种植被样本,主要是草和杂草,作为背景比较,分析了29种多氯联苯对二恶英(PCDDs),多氯二苯并呋喃(PCDF)和多氯联苯(PCB)。房屋周边植被样品的平均毒性当量(TEQ)为4.2至377 pg / g。 TEQs(植被与土壤)的比例约为0.3,最大值为3.5。根据土壤与植被之间同类模式的相似性计算,似乎植被污染源是周围的土壤。该结论得到线性回归分析的支持,线性回归分析表明,植被浓度log_(10)的结果变量对R〜2的最大贡献是周围土壤浓度的log_(10)。植被污染的模型通常侧重于大气沉积和分区。此处获得的结果表明,土壤颗粒在植被上的沉积是住宅用牧草污染的重要途径。因此,在受持久性有机化合物历史性工业排放影响的社区中,对污染性居民草本的准确建模至关重要,包括将土壤颗粒沉积到植被上至关重要。

著录项

  • 来源
    《Environmental toxicology and chemistry》 |2010年第12期|p.2660-2668|共9页
  • 作者单位

    Department of Civil and Environmental Engineering, University of Michigan College of Engineering, Ann Arbor, Michigan 48109, USA;

    LimnoTech, Ann Arbor, Michigan, USA;

    Department of Civil and Environmental Engineering, University of Michigan College of Engineering, Ann Arbor, Michigan 48109, USA;

    Department of Biostatistics, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Department of Environmental Health Sciences, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Department of Biostatistics, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Department of Environmental Health Sciences, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Department of Biostatistics, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Department of Environmental Health Sciences, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Department of Environmental Health Sciences, University of Michigan School of Public Health, Ann Arbor, Michigan, USA;

    Institute for Social Research, University of Michigan, Ann Arbor, Michigan, USA;

    Vista Analytical Laboratory, El Dorado Hills, California, USA;

    Vista Analytical Laboratory, El Dorado Hills, California, USA;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    polychlorinated dibenzo-p-dioxins; polychlorinated dibenzofurans; polychlorinated biphenyls; vegetation; soil;

    机译:多氯二苯并对二恶英;多氯二苯并呋喃;多氯联苯;植被;泥;

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