Selective excitation of the vibrational-rotational states and dissociation of diatomic molecules by picosecond infrared laser pulses: Modeling for HF in the ground electronic state

Andrianov IV.; Paramonov GK.

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Selective excitation of the vibrational-rotational states and dissociation of diatomic molecules by picosecond infrared laser pulses: Modeling for HF in the ground electronic state

机译：皮秒红外激光脉冲对振动旋转状态的选择性激发和双原子分子的解离：在基态电子状态下的HF建模

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Complete, close to 100%, population transfer between the bound vibrational-rotational states of the NF molecule in the ground electronic state is demonstrated on a picosecond time scale by means of computer simulation within the Schrodinger wave-function formalism. The laser-induced dissociation from selectively prepared moderately high vibrational-ratational states is shown to be very efficient, with the dissociation probability approaching 100%. These processes are controlled by sin(2)-shaped linearly polarized picosecond laser pulses in the infrared domain. [S1050-2947(99)05003-9]. [References: 20]

机译：通过在Schrodinger波函数形式主义内的计算机模拟，在皮秒级的时间尺度上证明了在基态电子状态下NF分子的束缚振动-旋转状态之间完整的，接近100％的种群转移。激光诱导的从选择性制备的中等高振动比状态下的解离非常有效，解离几率接近100％。这些过程由红外域中的sin（2）形线性偏振皮秒激光脉冲控制。 [S1050-2947（99）05003-9]。 [参考：20]

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《Physical Review, A. Atomic, molecular, and optical physics》 |1999年第3期|共5页
作者
Andrianov IV.; Paramonov GK.;
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正文语种 eng
中图分类物理学;
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Approximation; Environment;

机译：近似值;环境;

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1. Selective excitation of the vibrational-rotational states and dissociation of diatomic molecules by picosecond infrared laser pulses: Modeling for HF in the ground electronic state [J] . Andrianov IV., Paramonov GK. Physical Review, A. Atomic, molecular, and optical physics . 1999,第3期

机译：皮秒红外激光脉冲对振动旋转状态的选择性激发和双原子分子的解离：在基态电子状态下的HF建模
2. STATE-SELECTIVE CONTROL FOR VIBRATIONAL EXCITATION AND DISSOCIATION OF DIATOMIC MOLECULES WITH SHAPED ULTRASHORT INFRARED LASER PULSES [J] . Korolkov MV., Schmidt B., Paramonov GK. The Journal of Chemical Physics . 1996,第5期

机译：超短脉冲红外激光脉动分子的振动激发和解离的状态选择控制
3. Classical dynamics of multiphoton excitation and dissociation of diatomic molecules by infrared laser pulses [J] . Liu WK., Lin SH., Yuan JM. Physical Review, A. Atomic, molecular, and optical physics . 1999,第2期

机译：红外激光脉冲对双原子分子进行多光子激发和解离的经典动力学
4. Vibrationally State-Selective Electronic Excitation of Diatomic Molecules by Optimal Femtosecond Laser Pulses [C] . Korolkov, M.V., Paramonov, . 1998

机译：飞秒激光脉冲对双原子分子的振动态选择性电子激发
5. The Use of Ultrashort Picosecond Laser Pulses to Generate Quantum Optical Properties of Single Molecules in Biophysics. [D] . Ly, Sonny. 2012

机译：在生物物理学中使用超短皮秒激光脉冲生成单分子的量子光学性质。
6. Photoinduced refractive index variation within picosecond laser pulses excitation as the indicator of oxyorthosilicates single crystals composition modification [O] . Andrii V Uklein, Alexandr S Popov, Volodymyr V Multian, 2015

机译：皮秒激光脉冲激发下光诱导的折射率变化作为原硅酸单晶组成改性的指标
7. Electron excitation and 'cascade' ionisation of diatomic molecules with ultra-short pulses of strong IR lasers [O] . Pegarkov A. I. 2002

机译：双原子分子的电子激发和“级联”电离超强脉冲的强红外激光器
8. Theory of the Effects of Electronic Excitation on the Vibrational and Dissociative Relaxation of Diatomic Molecules. [R] . Taylor, D. K. 1966

机译：电子激发对双原子分子振动和解离弛豫影响的理论。

Selective excitation of the vibrational-rotational states and dissociation of diatomic molecules by picosecond infrared laser pulses: Modeling for HF in the ground electronic state

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