Striking AcOH Acceleration in Direct Intramolecular Allylic Amination Reactions

Fady Nahra; Frdric Liron; Guillaume Prestat; Carlo Mealli; Abdelatif Messaoudi; Giovanni Poli

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Striking AcOH Acceleration in Direct Intramolecular Allylic Amination Reactions

机译：直接分子内烯丙基胺化反应中惊人的AcOH加速

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Direct functionalisation of hydrocarbons has attracted much interest for its great potential in organic synthesis.[1] These processes, by avoiding the introduction of functional groups, have atom- and step-economical advantages. In this context, allylic functionalisation of olefins[2] is an active research domain, as witnessed by recent papers on Rh-,[3] Pd-[4] and Ru-catalysed[5] allylic acyloxylations and aminations of olefins.

机译：碳氢化合物的直接官能化因其在有机合成中的巨大潜力而吸引了很多兴趣。[1]这些方法通过避免引入官能团而具有原子和步骤经济的优势。在此背景下，烯烃的烯丙基官能化[2]是一个活跃的研究领域，最近有关Rh-，[3] Pd- [4]和Ru催化的[5]烯丙基酰化和烯烃胺化的论文证明了这一点。

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来源
《Chemistry: A European journal》 |2009年第42期|共5页
作者
Fady Nahra; Frdric Liron; Guillaume Prestat; Carlo Mealli; Abdelatif Messaoudi; Giovanni Poli;
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原文格式 PDF
正文语种 eng
中图分类应用化学;
关键词
AcOH; Direc; Intramolecular;

机译：AcOH;Direc;分子内;

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专利

1. Striking AcOH Acceleration in Direct Intramolecular Allylic Amination Reactions [J] . Fady Nahra, Freacute, deacute, Chemistry - A European Journal . 2010,第5期

机译：直接分子内烯丙基胺化反应中惊人的AcOH加速
2. Mechanistic Study of the Direct Intramolecular Allylic Amination Reaction Catalyzed by Palladium(II) [J] . Duarte Filipe J. S., Poli Giovanni, Calhorda Maria Jose ACS catalysis . 2016,第3期

机译：钯（II）催化直接分子内烯丙基胺化反应的机理研究
3. Hydroamination versus Allylic Amination in Iridium-Catalyzed Reactions of Allylic Acetates with Amines: 1,3-Aminoalcohols via Ester-Directed Regioselectivity [J] . SeungWook Kim, Thomas Wurm, Gilmar A. Brito, Journal of the American Chemical Society . 2018,第29期

机译：烯丙基乙酸与胺的铱催化反应中的氢化胺化与烯丙胺化反应：经由酯基区域选择性的1,3-氨基醇
4. Enantioselective Reactions of Bicyclic Allylic Compounds Based on Desymmetrization of a Symmetrical Allylic Ligand Using Chiral Palladium Complexes. [C] . Ryohei Ogawa, Yusuke Shigemori, Koichi Uehara Symposium on Organometallic Chemistry . 2006

机译：双环烯丙基化合物基于使用手性钯配合物的对称烯丙基配体的脱水化合物的映选择性反应。
5. Rhodium(I)-catalyzed allylic amination and carbocyclization reactions. [D] . Robinson, John E. 2004

机译：铑（I）催化的烯丙基胺化和碳环化反应。
6. Hydroamination versus Allylic Amination in Iridium Catalyzed Reactions of Allylic Acetates with Amines: 13-Aminoalcohols via Ester-Directed Regioselectivity [O] . Seung Wook Kim, Thomas Wurm, Gilmar A. Brito, -1

机译：铱催化烯丙乙酸酯与胺：13-氨基醇通过酯基定向区域选择性反应中的氢化胺化与烯丙胺化
7. Striking AcOH Acceleration in Direct Intramolecular Allylic Amination Reactions [O] . Fady Nahra, Frédéric Liron, Guillaume Prestat, 2010

机译：在直接分子内烯丙基胺化反应中醒目的acoh加速度
8. Reaction of Allylic and Benzylic Methyl Ethers with Sodium and Trimethylchlorosilane. Evidence for the Intermediacy of Allylic Radicals and Anions [R] . Tzeng, D., Weber, W. P. 1980

机译：烯丙基和苄基甲基醚与钠和三甲基氯硅烷的反应。烯丙基自由基和阴离子的中间性证据

Striking AcOH Acceleration in Direct Intramolecular Allylic Amination Reactions

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