SYNTHESIS OF THYMINE POLYOXIN C BY USING L-THREONINE ALDOLASE-CATALYZED ALDOL REACTION

Toshihiro Nishiyama; Swapnil Surendra Mohile; Tetsuya Kajimoto

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SYNTHESIS OF THYMINE POLYOXIN C BY USING L-THREONINE ALDOLASE-CATALYZED ALDOL REACTION

机译：L-苏氨酸醛糖酶催化的ALDOL反应合成胸苷多氧合酶C

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摘要

Thymine polyoxin C (2), a common partial structure of polyoxin H (3)and J (4)having anti-fungal activity, was formally synthesized from D-ribose in good overall yield by using L-threonine aldolase-catalyzed reaction as a key step, which affords novel beta-hydroxy-alpha-L-amino acids from glycine and aldehydes in an aqueous medium.

机译：通过L-苏氨酸醛缩酶催化的反应从D-核糖正式合成了胸腺嘧啶多氧信素C（2），它具有抗真菌活性。关键步骤，该步骤可在水性介质中从甘氨酸和醛中获得新的β-羟基-α-L-氨基酸。

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《Heterocycles: An International Journal for Reviews and Communications in Heterocyclic Chemistry》 |2007年第6期|共9页
作者
Toshihiro Nishiyama; Swapnil Surendra Mohile; Tetsuya Kajimoto;
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中图分类杂环化合物;
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1. SYNTHESIS OF THYMINE POLYOXIN C BY USING L-THREONINE ALDOLASE-CATALYZED ALDOL REACTION [J] . Toshihiro Nishiyama, Swapnil Surendra Mohile, Tetsuya Kajimoto Heterocycles: An International Journal for Reviews and Communications in Heterocyclic Chemistry . 2007,第6期

机译：L-苏氨酸醛糖酶催化的ALDOL反应合成胸苷多氧合酶C
2. A study towards efficient L-threonine aldolase-catalyzed enantio- and diastereoselective aldol reactions of glycine with substituted benzaldehydes: Biocatalyst production and process development [J] . Baer K., Dückers N., Rosenbaum T., Tetrahedron, Asymmetry: The International Journal for Repid Publication on all Aspects of Asymmetry in Orgainc, Inorganic, Organometallic, Physical and Bio-Organic Chemistry . 2011,第9期

机译：高效L-苏氨酸醛缩酶催化甘氨酸与取代的苯甲醛对映体和非对映体选择性醛醇缩合反应的研究：生物催化剂的生产和工艺开发
3. The first enantioselective synthesis of imino-deoxydigitoxose and protected imino-digitoxose by using L-threonine aldolase-catalyzed aldol condensation [J] . Nishiyama Toshihiro, Kajimoto Tetsuya, Mohile Swapnil S., Tetrahedron, Asymmetry: The International Journal for Repid Publication on all Aspects of Asymmetry in Orgainc, Inorganic, Organometallic, Physical and Bio-Organic Chemistry . 2009,第2期

机译：L-苏氨酸醛缩酶催化的醛醇缩合反应首次对映选择性合成亚氨基-脱氧数字氧糖和保护的亚氨基-数字氧糖
4. Germanium(II)-Mediated Reductive Cross-Aldol Reaction of Aldehydes:Synthesis of Aldols with Diastereocontrolled Quaternary Carbon Centers [C] . Shin-va Tanaka, Makoto Yasucla, Akio Baba Symposium on Organometallic Chemistry . 2007

机译：锗（II）膜的蛋白质介导的醛 - 醛醛 - 醛醇的合成与非杀螨科季碳中心合成
5. Strained silacycles in organic synthesis: The tandem aldol-allylatio/aldol-aldol reaction and their asymmetric variations. [D] . Wang, Xiaolun. 2005

机译：有机合成中的应变硅杂环化合物：串联的羟醛-烯丙基比/羟醛-羟醛反应及其不对称变化。
6. Comparison of L-Threonine Aldolase Variants in the Aldol and Retro-Aldol Reactions [O] . Kateryna Fesko 2019

机译：L-苏氨酸醛缩酶变体在醛醇和反醛醇反应中的比较。
7. Enhancement of the Diversity of Polyoxins by a Thymine-7-Hydroxylase Homolog outside the Polyoxin Biosynthesis Gene Cluster▿ † [O] . Zhao, Changming, Huang, Tingting, Chen, Wenqing, 2010

机译：胸腺嘧啶7-羟化酶同源物在多氧合蛋白生物合成基因簇外增强多氧合酶的多样性▿†

SYNTHESIS OF THYMINE POLYOXIN C BY USING L-THREONINE ALDOLASE-CATALYZED ALDOL REACTION

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