Allenes as three-carbon units in catalytic cycloadditions: New opportunities with transition-metal catalysts

L?pez F.; Mascare?as J.L.

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Allenes as three-carbon units in catalytic cycloadditions: New opportunities with transition-metal catalysts

机译：丙二烯在催化环加成中作为三碳单元：过渡金属催化剂的新机遇

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Allenes are very versatile synthetic units that are used in many types of catalytic cycloaddition reactions. Most examples reported so far involve their use as 2C-atom components, whereas their participations as 3C-atom components have been much less frequent. In this concept article, we present an overview of this latter strategy, emphasizing on those more recent contributions involving the use of Pt~(II) and Au~I catalysts, which have uncovered new opportunities in this area.

机译：丙二烯是非常通用的合成单元，用于许多类型的催化环加成反应中。到目前为止，大多数报道的例子都涉及将它们用作2C原子成分，而作为3C原子成分参与的频率则要低得多。在这一概念文章中，我们将对后一种策略进行概述，重点介绍那些最近在使用Pt〜（II）和Au〜I催化剂方面的贡献，这些发现为该领域带来了新的机遇。

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《Chemistry: A European journal》 |2011年第2期|共11页
作者
L?pez F.; Mascare?as J.L.;
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正文语种 eng
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关键词
allenes; cycloaddition; gold; homogeneous catalysis; synthetic methods;

机译：丙二烯;环加成;金;均相催化;合成方法;

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1. Allenes as three-carbon units in catalytic cycloadditions: New opportunities with transition-metal catalysts [J] . L?pez F., Mascare?as J.L. Chemistry: A European journal . 2011,第2期

机译：丙二烯在催化环加成中作为三碳单元：过渡金属催化剂的新机遇
2. Telomerization of 1,3-butadiene with various alcohols by Pd/TOMPP catalysts: new opportunities for catalytic biomass valorization [J] . Regina Palkovits, Andrei N. Parvulescu, Peter J. C. Hausoul Green chemistry . 2009,第8期

机译：Pd / TOMPP催化剂将1,3-丁二烯与各种醇进行端聚反应：催化生物质增值的新机会
3. Polysiloxanes in Catalysis and Catalyst Preparation: Opportunities for Control of Catalytic Processes [J] . Michael N. Missaghi, Mayfair C. Kung, Harold H. Kung Topics in Catalysis . 2012,第1a2期

机译：催化和催化剂制备中的聚硅氧烷：控制催化过程的机会
4. Molecular Basis for the Design of Transition-Metal Oxide Catalysts for Selective Catalytic Reduction of NO by Hydrocarbons [C] . K. Shimizu, H. Maeshima, H. Kawabata, International congress on catalysis;ICC . 2000

机译：设计用于烃选择性催化还原NO的过渡金属氧化物催化剂的分子基础
5. I. Photochemical catalytic [6pi + 2pi] higher-order cycloadditions. II. Toward the development of a chiral catalyst for chromium(0) higher-order cycloadditions. III. Synthetic studies toward a synthesis of taxol: Investigation of an intramolecular cycloaddition approach to the taxane core. [D] . Mann, Larry W. 2002

机译：I.光化学催化的[6pi + 2pi]高阶环加成。二。走向手性催化剂的铬（0）高阶环加成反应的发展。三，合成紫杉醇的合成研究：紫杉烷核心分子内环加成方法的研究。
6. Reactivityand Chemoselectivity of Allenes in Rh(I)-Catalyzed Intermolecular(5 + 2) Cycloadditions with Vinylcyclopropanes: Allene-Mediated RhodacycleFormation Can Poison Rh(I)-Catalyzed Cycloadditions [O] . Xin Hong, Matthew C. Stevens, Peng Liu, -1

机译：反应性（I）催化的分子间的异戊二烯的合成和化学选择性（5 + 2）与乙烯基环丙烷的环加成反应：丙二烯介导的Rhodacycle形成会毒化Rh（I）催化的环加成反应
7. Cycloadditions of Oxacyclic Allenes and a Catalytic Asymmetric Entryway to Enantioenriched Cyclic Allenes [O] . Michael M. Yamano, Rachel R. Knapp, Aurapat Ngamnithiporn, 2019

机译：氧化环烯族的环加成和对肾上腺环丙烯的催化不对称入口
8. Selective Catalytic Hydrogenation of Polynuclear Heteroaromatic Compounds Using Polymer-Supported Transition-Metal Compounds as Catalyst. [R] . Fish, R. H., Heinemann, H. 1985

机译：用聚合物负载的过渡金属化合物作催化剂选择性催化加氢多核杂芳族化合物。

Allenes as three-carbon units in catalytic cycloadditions: New opportunities with transition-metal catalysts

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