Ligand self-sorting and nonlinear effects in dinuclear asymmetric hydrogenation: Complexity in catalysis

Terrade F.G.; Lutz M.; Reek J.N.H.

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Ligand self-sorting and nonlinear effects in dinuclear asymmetric hydrogenation: Complexity in catalysis

机译：双核不对称加氢中的配体自分选和非线性效应：催化的复杂性

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Self-sorting species: Nonlinear effects are observed in asymmetric hydrogenation reactions if self-sorted dinuclear complexes are generated. The nature of the substrate also influences this effect, because it affects the solubility of racemic self-sorted homochiral dinuclear complexes (see scheme).

机译：自分选物种：如果产生了自分选的双核络合物，则会在不对称氢化反应中观察到非线性效应。底物的性质也会影响这种效果，因为它会影响外消旋的自分选同型手性双核复合物的溶解度（请参阅方案）。

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《Chemistry: A European journal》 |2013年第32期|共5页
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Terrade F.G.; Lutz M.; Reek J.N.H.;
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正文语种 eng
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asymmetric catalysis; complexity; hydrogenation; nonlinear effects; self-sorting;

机译：不对称催化复杂度加氢非线性效应自分选;

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1. Ligand self-sorting and nonlinear effects in dinuclear asymmetric hydrogenation: Complexity in catalysis [J] . Terrade F.G., Lutz M., Reek J.N.H. Chemistry: A European journal . 2013,第32期

机译：双核不对称加氢中的配体自分选和非线性效应：催化的复杂性
2. Enhancing Effects of Salt Formation on Catalytic Activity and Enantioselectivity for Asymmetric Hydrogenation of Isoquinolinium Salts by Dinuclear Halide-Bridged Iridium Complexes Bearing Chiral Diphosphine Ligands [J] . Kita Yusuke, Yamaji Kenta, Higashida Kosuke, Chemistry: A European journal . 2015,第5期

机译：盐形成对带有手性二膦配体的双核卤桥铱配合物对异喹啉鎓盐不对称加氢的催化活性和对映选择性的增强作用
3. Can a Butadiene-Based Architecture Compete with its Biaryl Counterpart in Asymmetric Catalysis? Enantiopure Me-CATPHOS, a Remarkably Efficient Ligand for Asymmetric Hydrogenation [J] . Doherty S, Smyth CH, Harriman A, Organometallics . 2009,第3期

机译：基于丁二烯的体系结构在不对称催化中能否与联芳基竞争？ Enantiopure Me-CATPHOS，非对称加氢的高效配体
4. Studies on Catalysis of Dinuclear Iridium Complexes with Bridging 1,4-Butadienyl Ligand [C] . Kohei Sasakura, Kazuhiro Okamoto, Kouichi Ohe 日本化学会春季年会講演予稿集 . 2018

机译：桥接1,4-丁二烯基配体催化二维铱络合物催化的研究
5. Metal-based asymmetric catalysis with N-heterocyclic carbene ligands, and, Lessons in asymmetric catalysis from a total synthesis of baconipyrone C. [D] . Gillingham, Dennis Gregory. 2007

机译：具有N-杂环卡宾配体的金属基不对称催化，以及从baconipyrone C的全合成获得的不对称催化的经验教训。
6. Asymmetric Catalysis Special Feature Part II: Remarkably diastereoselective synthesis of a chiral biphenyl diphosphine ligand and its application in asymmetric hydrogenation [O] . Liqin Qiu, Jing Wu, Shusun Chan, 2004

机译：不对称催化特征第二部分：手性联苯二膦配体的非对映选择性合成及其在不对称氢化中的应用
7. Cover Picture: Ligand Self-Sorting and Nonlinear Effects in Dinuclear Asymmetric Hydrogenation: Complexity in Catalysis (Chem. Eur. J. 32/2013) [O] . Frédéric G. Terrade, Martin Lutz, Joost N. H. Reek 2013

机译：封面图片：双核不对称氢化的配体自分排法和非线性效应：催化催化复杂性（Chem。欧元。J.32 / 2013）

Ligand self-sorting and nonlinear effects in dinuclear asymmetric hydrogenation: Complexity in catalysis

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