Hydroarylations of Heterobicyclic Alkenes through Rhodium-Catalyzed Directed C-H Functionalizations of S-Aryl Sulfoximines

Dong Wanrong; Parthasarathy Kanniyappan; Cheng Ying; Pan Fangfang; Bolm Carsten

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Hydroarylations of Heterobicyclic Alkenes through Rhodium-Catalyzed Directed C-H Functionalizations of S-Aryl Sulfoximines

机译：通过铑催化的S-芳基亚砜肟基的直接C-H官能团使杂环双环烯烃进行氢芳基化反应

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摘要

Rhodium-catalyzed directed CH-functionalizations have been used in hydroarylations of heterobicyclic alkenes with NH-sulfoximines. Unexpectedly, the bicyclic framework is retained, resulting in the formation of addition products being attractive intermediates for functionalized molecules that are difficult to prepare by other means.

机译：铑催化的定向CH-官能化已用于杂环双环烯烃与NH-亚砜肟的加氢芳基化反应。出乎意料的是，保留了双环骨架，导致形成加成产物，这是难以通过其他方式制备的官能化分子的有吸引力的中间体。

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《Chemistry: A European journal》 |2014年第48期|共5页
作者
Dong Wanrong; Parthasarathy Kanniyappan; Cheng Ying; Pan Fangfang; Bolm Carsten;
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正文语种 eng
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C-H activation; heterobicyclic alkenes; hydroarylation reaction; rhodium; sulfoximines;

机译：碳氢活化杂双环烯烃加氢芳基化反应铑亚砜;

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1. Hydroarylations of Heterobicyclic Alkenes through Rhodium-Catalyzed Directed C-H Functionalizations of S-Aryl Sulfoximines [J] . Dong Wanrong, Parthasarathy Kanniyappan, Cheng Ying, Chemistry: A European journal . 2014,第48期

机译：通过铑催化的S-芳基亚砜肟基的直接C-H官能团使杂环双环烯烃进行氢芳基化反应
2. Rhodium-catalyzed hydroarylation of alkynes via tetrazole-directed C-H activation [J] . Bin Chen, Yan Jiang, Jiang Cheng, Organic & biomolecular chemistry . 2015,第10期

机译：铑经四唑定向C-H活化的炔烃加氢芳基化反应
3. Amide-Directed Intramolecular Co(III)-Catalyzed C-H Hydroarylation of Alkenes for the Synthesis of Dihydrobenzofurans with a Quaternary Center [J] . Carral-Menoyo Asier, Sotomayor Nuria, Lete Esther The Journal of Organic Chemistry . 2020,第15期

机译：酰胺定向的分子内Co（III） - 烷烃的催化C-H加氢水合，用于合成二氢呋喃呋喃与第四纪中心
4. Rhodium-Catalyzed Intramolecular C-H Functionalization of Acceptor/acceptor Carbenoids Generated from 4-Acyl-1-sulfonyl-1,2,3-triazoles [C] . Qiang Zhao, Tomoya Miura, Masahiro Murakami 日本化学会春季年会講演予稿集 . 2018

机译：从4-酰基-1-磺酰基-1,2,3-三唑产生的受体/受体羧丙烯骨的铑催化的分子内C-H官能化
5. Copper-catalyzed functionalization of alkenes: Carboamination, C-H amination, C-H alkylation and carboetherifcation reactions. [D] . Liwosz, Timothy Walter. 2014

机译：铜催化烯烃的官能化：碳氨基化，C-H氨基化，C-H烷基化和碳醚化反应。
6. Rhodium-catalyzed asymmetric intramolecular hydroarylation of allenes: access to functionalized benzocycles [O] . Dino Berthold, Johannes Klett, Bernhard Breit 2019

机译：铑催化的烯基不对称分子内氢芳基化反应：获得功能化的苯并环
7. Enantioselective Intramolecular Hydroarylation of Alkenes via Directed C-H Bond Activation [O] . Harada, Hitoshi, Thalji, Reema, Bergman, Robert, 2008

机译：通过定向C-H键活化的烯烃的不对称分子内水解

Hydroarylations of Heterobicyclic Alkenes through Rhodium-Catalyzed Directed C-H Functionalizations of S-Aryl Sulfoximines

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