Palladium-Catalyzed Oxidative Synthesis of Highly Functionalized Ortholactones

Baddeley Kate L.; Cao Qun; Muldoon Mark J.; Cook Matthew J.

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Palladium-Catalyzed Oxidative Synthesis of Highly Functionalized Ortholactones

机译：钯催化氧化合成高官能度原内酯

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A palladium-catalyzed oxidative reaction is reported which converts dihydropyrans to their corresponding ortholactone. The products are formed in good to excellent yields with a very high level of chemoselectivity and functional group tolerance. Mechanistic studies confirm that the reaction proceeds by a Wacker-type mechanism.

机译：据报道钯催化的氧化反应将二氢吡喃转化为其相应的原内酯。形成的产品产率高至优异，具有很高的化学选择性和官能团耐受性。机理研究证实，反应是通过Wacker型机理进行的。

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《Chemistry: A European journal》 |2015年第21期|共5页
作者
Baddeley Kate L.; Cao Qun; Muldoon Mark J.; Cook Matthew J.;
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正文语种 eng
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关键词
aerobic oxidation; ortholactone; palladium; synthetic methods; Wacker-type reaction;

机译：好氧氧化;原内酯;钯;合成方法;Wacker型反应;

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专利

1. Palladium-Catalyzed Oxidative Synthesis of Highly Functionalized Ortholactones [J] . Baddeley Kate L., Cao Qun, Muldoon Mark J., Chemistry: A European journal . 2015,第21期

机译：钯催化氧化合成高官能度原内酯
2. Palladium-Catalyzed Four-Component Cascade Reaction for the Synthesis of Highly Functionalized Acyclic O,O-Acetals [J] . Wenfang Xiong, Donghao Yan, Chaorong Qi, Organic letters . 2018,第3期

机译：钯 - 催化的四组分级联反应用于合成高效官能化的无环，， O - 缩水
3. Palladium-catalyzed intermolecular tandem cyclization reaction: a highly regioselective synthesis of functionalized 3H-spiro [isobenzofuran-1,3'-isochroman] scaffolds [J] . Liang Wang, Xuehu Li, Hua Tao, Organic & biomolecular chemistry . 2017,第11期

机译：钯催化的分子间串联环化反应：高度区域选择性合成功能化的3H螺[异苯并呋喃-1,3'-异色满]支架。
4. Palladium-catalyzed acetic acid synthesis from methane and carbon dioxide [C] . Y.Fujiwara, Y.Taniguchi, K.Takaki, International natural gas conversion symposium . 1997

机译：钯催化的乙酸合成甲烷和二氧化碳
5. Palladium-catalyzed synthesis of heterocycles and highly functionalized polycyclics. [D] . Han, Xiaojun. 1998

机译：钯催化的杂环和高度官能化的多环化合物的合成。
6. Potassium Hydroxide Impregnated Alumina (KOH-Alumina) as a Recyclable Catalyst for the Solvent-Free Multicomponent Synthesis of Highly Functionalized Substituted Pyridazines and/or Substituted Pyridazin-3(2H)-ones under Microwave Irradiation [O] . Hormi Mecadon, Bekington Myrboh 2011

机译：微波辐射下氢氧化钾浸渍的氧化铝（KOH-氧化铝）作为无溶剂多组分合成高功能取代的哒嗪和/或取代的哒嗪-3（2H）-的可回收催化剂
7. Palladium-catalyzed synthesis of heterocycles and highly functionalized polycyclics [O] . Han, Xiaojun 1998

机译：钯催化的杂环和高度官能化的多环化合物的合成
8. Synthesis of Ceramics from Solutions: Functionally Graded Composites,NanoComposites and Single Crystal Thin Films. Epitaxial Growth and Structure of Highly Mismatched Oxide Films with Rock-Salt Structure on MgO [R] . Langjahr, P. A., Wagner, T., Lange, F. F., 1997

机译：从溶液中合成陶瓷：功能梯度复合材料，纳米复合材料和单晶薄膜。 mgO上岩盐结构高度错配氧化膜的外延生长和结构

Palladium-Catalyzed Oxidative Synthesis of Highly Functionalized Ortholactones

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