Electron-Accepting pi-Conjugated Molecules with Fluorine-Containing Dicyanovinylidene as Terminal Groups: Synthesis, Properties, and Semiconducting Characteristics

Ie Yutaka; Uchida Ayana; Kawaguchi Nana; Nitani Masashi; Tada Hirokazu; Kakiuchi Fumitoshi; Aso Yoshio

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Electron-Accepting pi-Conjugated Molecules with Fluorine-Containing Dicyanovinylidene as Terminal Groups: Synthesis, Properties, and Semiconducting Characteristics

机译：以含氟双氰基亚乙烯基为末端基团的电子接受π共轭分子：合成，性质和半导体特性

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A series of electron-accepting pi-conjugated molecules having fluorine-containing dicyanovinylidene as terminal groups has been synthesized for the application to electron-transporting semiconductors. This terminal group can be easily incorporated into pi-conjugated frameworks. Electrochemical measurements indicated that these compounds showed low-lying lowest unoccupied molecular orbital energy levels, which could be fine-tuned by the combination of central unit. The thin films fabricated by solution process showed typical electron-transporting characteristics in field-effect transistors.

机译：已经合成了一系列具有含氟二氰基亚乙烯基作为端基的电子接受性π-共轭分子，以用于电子传输半导体。该末端基团可以容易地掺入π-缀合的框架中。电化学测量表明，这些化合物显示出最低的最低未占据分子轨道能级，可以通过中央单元的组合进行微调。通过溶液工艺制备的薄膜在场效应晶体管中显示出典型的电子传输特性。

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《Organic letters》 |2016年第17期|共4页
作者
Ie Yutaka; Uchida Ayana; Kawaguchi Nana; Nitani Masashi; Tada Hirokazu; Kakiuchi Fumitoshi; Aso Yoshio;
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1. Electron-Accepting pi-Conjugated Molecules with Fluorine-Containing Dicyanovinylidene as Terminal Groups: Synthesis, Properties, and Semiconducting Characteristics [J] . Ie Yutaka, Uchida Ayana, Kawaguchi Nana, Organic letters . 2016,第17期

机译：以含氟双氰基亚乙烯基为末端基团的电子接受π共轭分子：合成，性质和半导体特性
2. Electron-Accepting pi-Conjugated Molecules with Fluorine-Containing Dicyanovinylidene as Terminal Groups: Synthesis, Properties, and Semiconducting Characteristics [J] . Ie Yutaka, Uchida Ayana, Kawaguchi Nana, Organic letters . 2016,第17期

机译：以含氟双氰基亚乙烯基为末端基团的电子接受π共轭分子：合成，性质和半导体特性
3. Synthesis, properties, and semiconducting characteristics of electron-transporting three-dimensional pi-conjugated compounds containing dicyanomethylene-substituted difluorocyclopenta[b]thiophene [J] . Ie Yutaka, Jinnai Seihou, Karakawa Makoto, Journal of Fluorine Chemistry . 2015,第Null期

机译：含二氰基亚甲基取代的二氟环戊[b]噻吩的电子传输三维π共轭化合物的合成，性质和半导体特性
4. Synthesis of pi-Conjugated Molecules via Rhodium-Carbene Complexes as Key Intermediates [C] . Tomohiro Abo, Koji Miki, Kouichi Ohe Symposium on Organometallic Chemistry . 2006

机译：通过铑 - 卡宾配合物合成PI缀合分子作为关键中间体
5. Synthesis and characterization of molecules and pi-conjugated materials containing low-coordinate phosphorus. [D] . Chen, Xufang. 2005

机译：含低配位磷的分子和pi共轭材料的合成与表征。
6. Synthesis and Regiochemistry of 60Fullerenyl 2-Methylmalonate Bisadducts and their Facile Electron-Accepting Properties [O] . Ken Kokubo, Riyah S. Arastoo, Takumi Oshima, -1

机译：合成和60 Fullerenyl 2-甲基丙Bisadducts及其简易电子接受性的区域化学
7. Synthesis, Molecular Packing, and Electrical Properties of New Regioisomeric ntype Semiconducting Molecules with Modification of Alkyl Substituents Position [O] . -1

机译：新型核苷酸半导体分子的合成，分子包装和电性能，改性烷基取代基位置
8. Synthesis and Properties of Semiconducting and Metallic Derivatives of Polyacetylene, (CH)x [R] . MacDiarmid, A. G., Heeger, A. J. 1978

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Electron-Accepting pi-Conjugated Molecules with Fluorine-Containing Dicyanovinylidene as Terminal Groups: Synthesis, Properties, and Semiconducting Characteristics

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