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Interparticle interactions: Energy potentials, energy transfer, and nanoscale mechanical motion in response to optical radiation

机译:粒子间相互作用:势能,能量转移和响应光辐射的纳米级机械运动

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摘要

In the interactions between particles of material with slightly different electronic levels, unusually large shifts in the pair potential can result from photoexcitation, and on subsequent electronic excitation transfer. To elicit these phenomena, it is necessary to understand the fundamental differences between a variety of optical properties deriving from dispersion interactions, and processes such as resonance energy transfer that occur under laser irradiance. This helps dispel some confusion in the recent literature. By developing and interpreting the theory at a deeper level, one can anticipate that in suitable systems, light absorption and energy transfer will be accompanied by significant displacements in interparticle separation, leading to nanoscale mechanical motion.
机译:在电子水平稍有不同的材料颗粒之间的相互作用中,光激发和随后的电子激发转移会导致线对电位发生异常大的变化。为了引起这些现象,有必要了解由色散相互作用产生的各种光学性质与诸如在激光辐照下发生的共振能量转移等过程之间的根本区别。这有助于消除最近文献中的一些混乱。通过更深入地发展和解释该理论,可以预期在合适的系统中,光吸收和能量转移将伴随着颗粒间分离的明显位移,从而导致纳米级机械运动。

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