Intense-Field Double Detachment of Electrostatically Bound F-(NF3)(n) Cluster Anions

Albeck Y.; Lerner G.; Kandhasamy D. M.; Chandrasekaran V.; Strasser D.

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Intense-Field Double Detachment of Electrostatically Bound F-(NF3)(n) Cluster Anions

机译：静电结合的F-（NF3）（n）团簇阴离子的强场双分离

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The interaction of intense laser pulses with size-selected F-(NF3)(n) clusters is experimentally studied. Intense-field double- and multiple-detachment processes in the isolated atomic F- anion and in electrostatically bound F-(NF3) dimer and F-(NF3)(2) trimer systems are directly compared. Both dimer and trimer systems are found to exhibit similar enhancement of the highly nonlinear processes, with respect to the atomic system, as reflected in significantly lower saturation intensities. The dependencies of different product channels as, a function of laser peak intensity, polarization ellipticity, and laser pulse shape are presented, indicating an efficient nonrescattering mechanism.

机译：实验研究了强激光脉冲与尺寸选择的F-（NF3）（n）团簇的相互作用。直接比较了孤立原子中的F-阴离子和静电结合的F-（NF3）二聚体和F-（NF3）（2）三聚体系统中的强场双离和多次分离过程。发现二聚体系统和三聚体系统相对于原子系统都表现出高度非线性过程的相似增强，这反映在明显较低的饱和强度上。给出了不同产品通道的依赖性，这些依赖性是激光峰值强度，偏振椭圆率和激光脉冲形状的函数，表明了一种有效的非散射机制。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2016年第19期|共7页
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Albeck Y.; Lerner G.; Kandhasamy D. M.; Chandrasekaran V.; Strasser D.;
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1. Intense-Field Double Detachment of Electrostatically Bound F-(NF3)(n) Cluster Anions [J] . Albeck Y., Lerner G., Kandhasamy D. M., The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2016,第19期

机译：静电结合的F-（NF3）（n）团簇阴离子的强场双分离
2. Decays of excited silver-cluster anions Ag_n, n = 4 to 7, in the Double ElectroStatic Ion Ring ExpEriment [J] . E. K. Anderson, M. Kamińska, K. C. Chartkunchand, Physical Review, A . 2018,第2aPta1期

机译：在双静电离子环实验中衰变激动的银簇阴离子Ag_n，n = 4至7
3. Electron binding energies of dipole-bound anions at the coupled cluster level with single, double, and triple excitations: HCN~- and HNC~- [J] . Kirk A.Peterson, Maciej Gutowski The Journal of Chemical Physics . 2002,第8期

机译：单，双和三激发在偶合簇能级上偶极结合阴离子的电子结合能：HCN〜-和HNC〜-
4. Electron Detachment Dissociation of Anion-Adducted Peptides [C] . Tao Jiang, Kristina Hakansson American Society for Mass Spectrometry Conference on Mass Spectrometry and Allied Topics . 2013

机译：电子脱离阴离子加入肽解离
5. Anion photoelectron spectroscopic and reactivity studies of gas phase biomolecules, diffusely bound electron states, aluminum clusters, and rare earth doped silicon clusters. [D] . Stokes, Sarah Tomlinson. 2008

机译：气相生物分子，弥散键合电子态，铝簇和稀土掺杂硅簇的阴离子光电子能谱和反应性研究。
6. Electrostatic properties of the anion selective porin Omp32 from Delftia acidovorans and of the arginine cluster of bacterial porins [O] . Ulrich Zachariae, Assen Koumanov, Harald Engelhardt, 2002

机译：Delftia acidovorans的阴离子选择性孔蛋白Omp32和细菌孔蛋白精氨酸簇的静电性质
7. Decays of excited silver-cluster anions Agn , n=4 to 7, in the Double ElectroStatic Ion Ring ExpEriment [O] . E. K. Anderson, M. Kamińska, K. C. Chartkunchand, 2018

机译：在双静电离子环实验中衰减兴奋的银色簇阴离子AgN，n = 4至7，
8. Product Vibrational State Distributions in Thermal Energy Associative Detachment Reactions: F- + H,D Yields HF(v), DF(v) + e-. [R] . Smith, M. A., Leone, S. R. 1983

机译：热能缔合分离反应中的产物振动状态分布：F- + H，D产率HF（v），DF（v）+ e-。

Intense-Field Double Detachment of Electrostatically Bound F-(NF3)(n) Cluster Anions

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