Control over the preference for binding sites of polyoxometalates to silver ethynide clusters by surface charge modification

Tamari Sho; Ono Kosuke; Hashimoto Masato; Ozeki Tomoji

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Control over the preference for binding sites of polyoxometalates to silver ethynide clusters by surface charge modification

机译：通过表面电荷修饰控制多金属氧酸盐与乙炔银簇结合位点的偏好

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A polyoxometalate-silver ethynide composite cluster, [Ag-42(CO3)-{ C = CC(CH3)(3)}(27)(alpha-A-SiW9Nb3O40)(2)](-) (1), demonstrates that we can select the binding site of a polyoxometalate to the silver alkynide cluster by tuning the surface charge of the precursor polyoxometalate. Multidimensional and multinuclear NMR spectra revealed that 1 maintains its precise atomic connectivity in the solution.

机译：多金属氧酸盐-乙炔银复合簇[Ag-42（CO3）-{C = CC（CH3）（3）}（27）（alpha-A-SiW9Nb3O40）（2）]（-）（1）证明我们可以通过调节多金属氧酸盐前体的表面电荷来选择多金属氧酸盐与炔银簇的结合位点。多维和多核NMR光谱显示1在溶液中保持其精确的原子连通性。

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《Dalton transactions: An international journal of inorganic chemistry》 |2015年第44期|共3页
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Tamari Sho; Ono Kosuke; Hashimoto Masato; Ozeki Tomoji;
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1. Control over the preference for binding sites of polyoxometalates to silver ethynide clusters by surface charge modification [J] . Tamari Sho, Ono Kosuke, Hashimoto Masato, Dalton transactions: An international journal of inorganic chemistry . 2015,第44期

机译：通过表面电荷修饰控制多金属氧酸盐与乙炔银簇结合位点的偏好
2. Anion Templated Synthesis of Silver(I)-Ethynide Dithiophosphate Clusters [J] . Jin Jun-Ling, Shen Yang-Lin, Xie Yun-Peng, Nature reviews Cancer . 2018,第8期

机译：银（I）的阴离子模板合成 - 丙酰胺二硫代磷酸簇
3. High- nuclearity silver ethynide clusters containing polynucleating oxygen donor ligands [J] . Jin Jun-Ling, Xie Yun-Peng, Lu Xing Dalton transactions: An international journal of inorganic chemistry . 2018,第37期

机译：含有多核氧供体配体的高核酸银簇簇
4. Electrochemistry, Spectrophotometry, and NMR Investigations of Chemisorption of Polyoxometalate on Silver Nanoparticle Surfaces [C] . G. C. Lica, B. S. Zelakiewicz, L. Smeeding ECS Meeting . 2003

机译：电化学，分光光度法和NMR研究银纳米粒子表面上多氧酸盐酸盐的研究
5. Reaction of aqueous polyoxometalates with silver and gold surfaces. [D] . Powell, Jason Daniel. 2001

机译：水性多金属氧酸盐与银和金表面的反应。
6. Conserved Surface-Exposed K/R-X-K/R Motifs and Net Positive Charge on Poxvirus Complement Control Proteins Serve as Putative Heparin Binding Sites and Contribute to Inhibition of Molecular Interactions with Human Endothelial Cells: a Novel Mechanism for Evasion of Host Defense [O] . Scott A. Smith, Nick P. Mullin, John Parkinson, 2000

机译：保守的表面暴露的K / R-X-K / R母体和痘病毒补体控制蛋白上的净正电荷作为推定的肝素结合位点发挥作用并有助于抑制与人类内皮细胞的分子相互作用：规避宿主防御的新机制
7. Conserved Surface-Exposed K/R-X-K/R Motifs and Net Positive Charge on Poxvirus Complement Control Proteins Serve as Putative Heparin Binding Sites and Contribute to Inhibition of Molecular Interactions with Human Endothelial Cells: a Novel Mechanism for Evasion of Host Defense [O] . Smith, Scott A., Mullin, Nick P., Parkinson, John, 2000

机译：保守的表面暴露的K / R-X-K / R母体和痘病毒补体控制蛋白上的净正电荷作为推定的肝素结合位点发挥作用，并有助于抑制与人类内皮细胞的分子相互作用：规避宿主防御的新机制

Control over the preference for binding sites of polyoxometalates to silver ethynide clusters by surface charge modification

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