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Effects of growth temperature and thermal annealing on optical quality of GaNAs nanowires emitting in the near-infrared spectral range

机译:生长温度和热退火对近红外光谱范围发射GANAS纳米线光学质量的影响

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We report on optimization of growth conditions of GaAs/GaNAs/GaAs core/shell/shell nanowire (NW) structures emitting at similar to 1 mu m, aiming to increase their light emitting efficiency. A slight change in growth temperature is found to critically affect optical quality of the active GaNAs shell and is shown to result from suppressed formation of non-radiative recombination (NRR) centers under the optimum growth temperature. By employing the optically detected magnetic resonance spectroscopy, we identify gallium vacancies and gallium interstitials as being among the dominant NRR defects. The radiative efficiency of the NWs can be further improved by post-growth annealing at 680 degrees C, which removes the gallium interstitials.
机译:我们报告了GaAs / GANAS / GAAs /壳/壳/壳纳米线(NW)结构的增长条件的优化报告,其在类似于1μm的情况下发射,旨在提高其发光效率。 发现生长温度的微小变化是影响活性GANAS壳的光学质量,并显示出在最佳生长温度下抑制非辐射重组(NRR)中心的形成。 通过采用光学检测的磁共振光谱,我们鉴定镓空位和镓间质缺乏症是主要的NRR缺陷中。 通过在680℃的680℃下的生长后退火可以进一步提高NWS的辐射效率,从而除去镓间质性。

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