Metal-free oxidative isocyanides insertion with aromatic aldehydes to aroylated N-heterocycles

He Yimiao; Wang Xuelian; Xiao Jun-An; Pang Jinying; Gan Chunfang; Huang Yanmin; Huang Chusheng

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Metal-free oxidative isocyanides insertion with aromatic aldehydes to aroylated N-heterocycles

机译：无金属氧化异氰化物与芳香醛插入芳香族醛基氧化N-杂环

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A metal-free, mild and efficient protocol for the construction of aroylated N-heterocycles via radical cascade aroylation of phenyl or vinyl isocyanides with aromatic aldehydes has been developed. Both phenanthridine and isoquinoline derivatives are delivered quickly in moderate to good yields with high regioselectivity.

机译：已经开发了一种通过自由基级联苯基或乙烯基异氰酸酯与芳香族醛植物构建的无金属，温和和高效的方案的亚氧化N-杂环。菲利丁和异喹啉衍生物均以高度的高产量迅速递送，具有高区域选择性。

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来源
《RSC Advances》 |2018年第6期|共5页
作者
He Yimiao; Wang Xuelian; Xiao Jun-An; Pang Jinying; Gan Chunfang; Huang Yanmin; Huang Chusheng;
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作者单位

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

Guangxi Teachers Educ Univ Coll Chem &

Mat Sci Nanning 530001 Peoples R China;

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正文语种 eng
中图分类化学;
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1. Metal-free oxidative isocyanides insertion with aromatic aldehydes to aroylated N-heterocycles [J] . He Yimiao, Wang Xuelian, Xiao Jun-An, RSC Advances . 2018,第6期

机译：无金属氧化异氰化物与芳香醛插入芳香族醛基氧化N-杂环
2. Sulfuric Acid-Promoted Oxidation of Benzylic Alcohols to Aromatic Aldehydes in Dimethyl Sulfoxide: An Efficient Metal-Free Oxidation Approach [J] . Sheikhi Ehsan, Adib Mehdi, Karajabad Morteza Akherati, Synlett . 2018,第7期

机译：硫酸 - 促进苄醇氧化在二甲基亚甲醚中的芳族醛：无需无金属氧化方法
3. Zinc Chloride Promoted Formal Oxidative Coupling of Aromatic Aldehydes and Isocyanides to r-Ketoamides [J] . Marinus Bouma, Geraldine Masson, Jieping Zhu The Journal of Organic Chemistry . 2010,第8期

机译：氯化锌促进芳族醛和异氰酸酯与r-酮酰胺的形式氧化偶合
4. Enzymatic hydrolysis lignin oxidation to prepare aromatic aldehydes with activation of Fenton reagent [C] . Zhen Wu, Ning Xu, Lei Hu International Conference on Energy and Environmental Protection . 2014

机译：酶水解木质素氧化用芬顿试剂的活化制备芳香族醛
5. Bulk gold catalyzed oxidation reactions of amines and isocyanides and iron porphyrin catalyzed N-H and O-H bond insertion/cyclization reactions of diamines and aminoalcohols [D] . Klobukowski, Erik Richard 2011

机译：胺和异氰化物的体金催化氧化反应和铁卟啉催化的二胺和氨基醇的N-H和O-H键插入/环化反应
6. An Oxidation of Benzyl Methyl Ethers with NBS that Selectively Affords Either Aromatic Aldehydes or Aromatic Methyl Esters [O] . Abdelrahman S. Mayhoub, Arindam Talukdar, Mark Cushman -1

机译：甲基苄醚与NBs选择性得到无论是芳香醛或芳香甲酯的氧化
7. Metal-free oxidative isocyanides insertion with aromatic aldehydes to aroylated N-heterocycles [O] . Yimiao He, Xuelian Wang, Jun-An Xiao, 2018

机译：无金属氧化异氰化物与芳香醛插入芳香族醛基氧化N-杂环
8. Metalation of Heterocyclic Aromatic Aldehydes Directed by Alpha-Amino Alkoxides [R] . Killpack, M. O. 1985

机译：α-氨基醇盐指导的杂环芳香醛的金属化

Metal-free oxidative isocyanides insertion with aromatic aldehydes to aroylated N-heterocycles

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