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Highly conductive carbon-based aqueous inks toward electroluminescent devices, printed capacitive sensors and flexible wearable electronics

机译:高导电碳基含水油墨朝向电致发光器件,印刷电容传感器和灵活的可穿戴电子产品

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摘要

Carbon-based conductive inks are one of the most important materials in the field of printing electronics. However, most carbon-based conductive inks with small electrical resistance are expensive, such as graphene. It limits the commercial use of carbon inks in the fields of flexible electronics and printed electronics. Here, we propose a low-cost and environmentally friendly formula based on dihydroxyphenyl-functionalized multi-walled carbon nanotubes (MWNT-f-OH)/carbon black/graphite as conductive fillers and waterborne acrylic resins as binders for preparing highly conductive carbon-based aqueous inks (HCCA-inks). Our study showed that when the mass fraction of carbon black, graphite and MWNT-f-OH was 3.0%, 10.2% and 4.1%, respectively, on a thickness of 40 m, optimal conductivity (sheet resistance up to 29 sq(-1)) was achieved, and the printed HCCA-inks on a paper could withstand extremely high folding cycles (>2000 cycles) while the resistance value of the flexible circuit only increased by 11%. The carbon-based aqueous inks showed high electrical conductivity and excellent mechanical stability, which makes it possible for them to be used as flexible wearable electronics, electroluminescent (EL) devices and printed capacitive sensors.
机译:碳的导电油墨是印刷电子领域中最重要的材料之一。然而,具有小电阻的大多数基于碳的导电油墨是昂贵的,例如石墨烯。它限制了柔性电子和印刷电子领域的碳油墨的商业用途。在这里,我们提出了基于二羟基苯基官能化的多壁碳纳米管(MWNT-F-OH)/炭黑/石墨作为导电填料和水性丙烯酸树脂作为用于制备高导电性碳的粘合剂的低成本和环保的配方含水油墨(HCCA-LICKS)。我们的研究表明,当炭黑,石墨和MWNT-F-OH的质量分数分别为3.0%,10.2%和4.1%,厚度为40μm,最佳导电性(薄层电阻高达29平方Sq(-1) ))实现,纸上的印刷HCCA-油墨可以承受极高的折叠循环(> 2000个循环),而柔性电路的电阻值仅增加11%。碳基含水油墨显示出高导电性和优异的机械稳定性,这使得它们可以用作柔性可佩戴电子设备,电致发光(EL)器件和印刷电容传感器。

著录项

  • 来源
    《RSC Advances》 |2019年第27期|共6页
  • 作者单位

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

    Yale Univ Sch Engn &

    Appl Sci Chem &

    Environm Engn 17 Hillhouse Ave New Haven CT 06511 USA;

    Yale Univ Sch Engn &

    Appl Sci Chem &

    Environm Engn 17 Hillhouse Ave New Haven CT 06511 USA;

    Wuhan Univ Sch Printing &

    Packaging Luojia Hill Wuhan 430072 Hubei Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 化学;
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