Design, synthesis, characterization, and catalytic properties of a large-pore metal-organic framework possessing single-site vanadyl(monocatecholate) moieties

Nguyen H.G.T.; Weston M.H.; Sarjeant A.A.; Gardner D.M.; An Z.; Carmieli R.; Wasielewski M.R.; Farha O.K.; Hupp J.T.; Nguyen S.T.

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Design, synthesis, characterization, and catalytic properties of a large-pore metal-organic framework possessing single-site vanadyl(monocatecholate) moieties

机译：具有单位钒酸单儿茶酚酯部分的大孔金属有机骨架的设计，合成，表征和催化性能

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Through a combination of protecting groups, postsynthesis deprotection, and postsynthesis metallation, a homogeneously inaccessible, single-site vanadyl(monocatecholate) moiety can be incorporated into the dipyridyl struts of a Zn-based, pillared paddlewheel MOF. The resulting MOF, which has large pores, exhibits catalytic activity in the benzylic oxidation of tetralin in the presence of tert-butylhydroperoxide.

机译：通过保护基团的组合，合成后的去保护和合成后的金属化，可以将均一且难以接近的单部位钒基（单儿茶酚酸酯）部分结合到Zn基柱状桨式MOF的二吡啶基撑杆中。所得的具有大孔的MOF在叔丁基过氧化氢的存在下在四氢化萘的苄基氧化中表现出催化活性。

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《Crystal growth & design》 |2013年第8期|共7页
作者
Nguyen H.G.T.; Weston M.H.; Sarjeant A.A.; Gardner D.M.; An Z.; Carmieli R.; Wasielewski M.R.; Farha O.K.; Hupp J.T.; Nguyen S.T.;
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正文语种 eng
中图分类 54.9;
关键词
large-pore metal-organic; framework possessing; moieties;

机译：大孔金属有机物;框架占有;部分;

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1. Design, synthesis, characterization, and catalytic properties of a large-pore metal-organic framework possessing single-site vanadyl(monocatecholate) moieties [J] . Nguyen H.G.T., Weston M.H., Sarjeant A.A., Crystal growth & design . 2013,第8期

机译：具有单位钒酸单儿茶酚酯部分的大孔金属有机骨架的设计，合成，表征和催化性能
2. Design, synthesis and characterization of a Pt-Gd metal-organic framework containing potentially catalytically active sites [J] . Szeto KC, Kongshaug KO, Jakobsen S, Dalton transactions: An international journal of inorganic chemistry . 2008,第15期

机译：包含潜在催化活性位点的Pt-Gd金属有机骨架的设计，合成和表征
3. Design, synthesis and characterization of a Pt-Gd metal-organic framework containing potentially catalytically active sites [J] . Kai C. Szeto, Kjell Ove Kongshaug, Soren Jakobsen Dalton transactions: An international journal of inorganic chemistry . 2008,第15期

机译：包含潜在催化活性位点的Pt-Gd金属有机骨架的设计，合成和表征
4. Synthesis of Metal-Organic Framework-Derived Carbon Supported CoFe_2O_4 with Enhanced Oxygen Reduction Reaction Catalytic Properties [C] . Zongzhao Li, Jing Sui, Qian Zhang, Pacific Rim Meeting on Electrochemical and Solid-State Science . 2020

机译：用增强的氧还原反应催化性能合成金属 - 有机骨架衍生碳负载的COFE_2O_4
5. Design, synthesis, characterization, and sorption properties of metal-organic frameworks and polyhedra based on [iron(3)oxide(R dioxide)(6)L(3)](0/+) clusters. [D] . Sudik, Andrea C. 2005

机译：设计，合成，表征，和基于[铁（3）氧化物（R二氧化）（6）L（3）]（0 / +）簇的多面体的吸附性能。
6. Metal-Organic Frameworks to Metal/Metal Oxide Embedded Carbon Matrix: Synthesis Characterization and Gas Sorption Properties [O] . Jiun-Jen Chen, Ya-Ting Chen, Duraisamy Senthil Raja, 2015

机译：金属/金属氧化物嵌入的碳基体的金属有机骨架：合成表征和气体吸附性能
7. Synthesis, characterization, adsorption and catalytic properties of an amino functionalized Metal-Organic Framework: NH2-MIL-47 [O] . Leus Karen, Couck S, Bogaerts Thomas, 2012

机译：氨基官能化金属有机骨架的合成，表征，吸附和催化性能：NH2-mIL-47

Design, synthesis, characterization, and catalytic properties of a large-pore metal-organic framework possessing single-site vanadyl(monocatecholate) moieties

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