In situ Raman Quantitative Detection of the Cold Seep Vents and Fluids in the Chemosynthetic Communities in the South China Sea

Du Zengfeng; Zhang Xin; Luan Zhendong; Wang Minxiao; Xi Shichuan; Li Lianfu; Wang Bing; Cao Lei; Lian Chao; Li Chaolun; Yan Jun

摘要

Abstract > Based on the previously developed deep‐sea hybrid Raman insertion probe for cold seeps, the in situ detection of a cold seep vent and geochemistry analysis of fluids in chemosynthetic communities were conducted at the Formosa Ridge in the northern South China Sea. Three different methods were used to measure the components of the fluids erupting from the cold seep vent. The in situ Raman spectra of the cold seep fluids indicated the presence of gaseous CH <sub>4</sub> , C <sub>3</sub> H <sub>8</sub> , and H <sub>2</sub> S. The results indicate that the gases at this site are of biogenic origin; however, the presence of C <sub>3</sub> H <sub>8</sub> suggests that thermogenic methane should not be excluded. The conclusion is also supported by the results of gas chromatography and stable carbon isotope analysis. More significantly, we found that the concentration of SO <sub>4</sub> 2? decreases with increasing depth, while the concentrations of CH <sub>4</sub> and S <sub>8</sub> increase in fluids in chemosynthetic communities, but without H <sub>2</sub> S. This finding indicates that the methane is oxidized by sulfate and that elemental sulfur is formed. This process usually occurs in marine sediments as the anaerobic oxidation of methane. Overall, the findings in this work provide a new insight into the geochemical analysis of cold seep fluids and in situ evidence of the oxidation of methane in the chemosynthetic communities near cold seeps. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 基于先前发育的深海杂交拉曼插入探针，用于冷渗透，在南海北部的福尔摩沙山脊上进行了调节社区中液体的冷渗透和地球化学分析的原位检测。使用三种不同的方法来测量从冷渗透发泄爆发的流体的组分。冷渗漏的原位拉曼光谱表明存在气态CH <sub> 4 </ sub> ， C <sub> 3 </ sub> H <sub> 8 </ sub> 和h. <sub> 2 </ sub> S.结果表明该网站的气体是生物起源的;但是，C的存在 <sub> 3 </ sub> H <sub> 8 </ sub> 表明不应排除热原甲烷。结论也得到了气相色谱和稳定的碳同位素分析的结果。更重要的是，我们发现所以的浓度 <sub> 4 </ sub> 2？</ sup> 随着深度的增加而降低，而CH的浓度 <sub> 4 </ sub> 和s <sub> 8 </ sub> 化学社区中的液体增加，但没有h <sub> 2 </ sub> S.该发现表明甲烷通过硫酸盐氧化，形成元素硫。该过程通常发生在海洋沉积物中作为甲烷的厌氧氧化。总体而言，这项工作中的调查结果对冷渗流的地球化学分析以及原位证据提供了新的探讨了在冷渗透附近的化学合作中甲烷氧化的原因。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23285/'>《Geochemistry, geophysics, geosystems》</a> <b style="margin: 0 2px;">|</b><span>2018年第7期</span><b style="margin: 0 2px;">|</b><span>共13页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Zengfeng&option=202" target="_blank" rel="nofollow">Du Zengfeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xin&option=202" target="_blank" rel="nofollow">Zhang Xin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Luan Zhendong&option=202" target="_blank" rel="nofollow">Luan Zhendong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Minxiao&option=202" target="_blank" rel="nofollow">Wang Minxiao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xi Shichuan&option=202" target="_blank" rel="nofollow">Xi Shichuan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Lianfu&option=202" target="_blank" rel="nofollow">Li Lianfu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Bing&option=202" target="_blank" rel="nofollow">Wang Bing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Lei&option=202" target="_blank" rel="nofollow">Cao Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lian Chao&option=202" target="_blank" rel="nofollow">Lian Chao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Chaolun&option=202" target="_blank" rel="nofollow">Li Chaolun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Jun&option=202" target="_blank" rel="nofollow">Yan Jun;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Raman spectroscopy&option=203" rel="nofollow">Raman spectroscopy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=in situ detection&option=203" rel="nofollow">in situ detection;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=cold seep fluids&option=203" rel="nofollow">cold seep fluids;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=chemosynthetic communities&option=203" rel="nofollow">chemosynthetic communities;</a> </p> <div class="translation"> 机译：拉曼光谱;原位检测;冷渗漏液;化学社区; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023360790.html">In situ Raman Quantitative Detection of the Cold Seep Vents and Fluids in the Chemosynthetic 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