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Ordered Arrangement and Optical Properties of Silica‐Stabilized Gold Nanoparticle–PNIPAM Core–Satellite Clusters for Sensitive Raman Detection

机译：二氧化硅稳定金纳米粒子-1PNIPAM芯卫星颗粒的有序布置和光学性质，用于敏感拉曼检测

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Abstract > Gold–polymer hybrid nanoparticles attract wide interest as building blocks for the engineering of photonic materials and plasmonic (active) metamaterials with unique optical properties. In particular, the coupling of the localized surface plasmon resonances of individual metal nanostructures in the presence of nanometric gaps can generate highly enhanced and confined electromagnetic fields, which are frequently exploited for metal‐enhanced light–matter interactions. The optical properties of plasmonic structures can be tuned over a wide range of properties by means of their geometry and the size of the inserted nanoparticles as well as by the degree of order upon assembly into 1D, 2D, or 3D structures. Here, the synthesis of silica‐stabilized gold–poly(N‐isopropylacrylamide) (SiO <sub>2</sub> ‐Au‐PNIPAM) core–satellite superclusters with a narrow size distribution and their incorporation into ordered self‐organized 3D assemblies are reported. Significant alterations of the plasmon resonance are found for different assembled structures as well as strongly enhanced Raman signatures are observed. In a series of experiments, the origin of the highly enhanced signals can be assigned to the interlock areas of adjacent SiO <sub>2</sub> ‐Au‐PNIPAM core–satellite clusters and their application for highly sensitive nanoparticle‐enhanced Raman spectroscopy is demonstrated. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> > gold-聚合物杂交纳米粒子吸引了具有独特光学性质的光子材料和等离子体（活性）超材料的构建块的广泛兴趣。特别地，各个金属纳米结构在纳米间隙存在下的局部表面等离子体谐振的耦合可以产生高度增强和狭窄的电磁场，其经常被利用用于金属增强的浅型相互作用。等离子体结构的光学性能可以通过它们的几何形状和插入的纳米颗粒的尺寸以及装配到1D，2D或3D结构时的顺序的宽度和尺寸在宽范围的性质上调。这里，二氧化硅稳定的金 - 聚（N-异丙基丙烯酰胺）的合成（SiO <sub> 2 </ sub> -u-pnipam）的核卫星超级全级，尺寸分布窄，并将其融入有序的自组织3D组件中据报道。对不同组装的结构的不同，等离子体谐振的显着改变以及观察到强大的拉曼签名。在一系列实验中，可以将高度增强信号的起源分配给相邻SiO <sub> 2 </ sub> -au-pnipam核心卫星簇的互锁区域及其对高敏感纳米颗粒增强的拉曼光谱的应用被证明。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-28247/'>《Small》</a> <b style="margin: 0 2px;">|</b><span>2017年第39期</span><b style="margin: 0 2px;">|</b><span>共1页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Herrmann Janning F.&option=202" target="_blank" rel="nofollow">Herrmann Janning F.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kretschmer Florian&option=202" target="_blank" rel="nofollow">Kretschmer Florian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hoeppener Stephanie&option=202" target="_blank" rel="nofollow">Hoeppener Stephanie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=H?ppener Christiane&option=202" target="_blank" rel="nofollow">H?ppener Christiane;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Schubert Ulrich S.&option=202" target="_blank" rel="nofollow">Schubert Ulrich S.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>NanobiophotonicsUniversity of MünsterWillhelm‐Klemm‐Str. 10 48149 Münster Germany;</p> <p>Laboratory of Organic and Macromolecular Chemistry (IOMC)Friedrich Schiller University JenaHumboldtstr. 10 07743 Jena Germany;</p> <p>Laboratory of Organic and Macromolecular Chemistry (IOMC)Friedrich Schiller University JenaHumboldtstr. 10 07743 Jena Germany;</p> <p>NanobiophotonicsUniversity of MünsterWillhelm‐Klemm‐Str. 10 48149 Münster Germany;</p> <p>Laboratory of Organic and Macromolecular Chemistry (IOMC)Friedrich Schiller University JenaHumboldtstr. 10 07743 Jena Germany;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=3D‐arrays&option=203" rel="nofollow">3D‐arrays;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=core–satellite nanoparticles&option=203" rel="nofollow">core–satellite nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal–polymer hybrid nanoparticles&option=203" rel="nofollow">metal–polymer hybrid nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoparticle‐enhanced Raman spectroscopy&option=203" rel="nofollow">nanoparticle‐enhanced Raman spectroscopy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=poly‐(N‐isopropyl acrylamide)&option=203" rel="nofollow">poly‐(N‐isopropyl acrylamide);</a> </p> <div class="translation"> 机译：3D阵列;核卫星纳米颗粒;金属 - 聚合物杂交纳米颗粒;纳米粒子增强拉曼光谱;聚 - （N-异丙基丙烯酰胺）; 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