Direct Functionalization of C-H Bonds by Iron, Nickel, and Cobalt Catalysis

Gerit Pototschnig; Nuno Maulide; Michael Schnerch

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Direct Functionalization of C-H Bonds by Iron, Nickel, and Cobalt Catalysis

机译：铁，镍和钴催化的C-H键直接官能化

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Non-precious-metal-catalyzed reactions are of increasing importance in chemistry due to the outstanding ecological and economic properties of these metals. In the subfield of metal-catalyzed direct C-H functionalization reactions, recent years have shown an increasing number of publications dedicated to this topic. Nickel, cobalt, and last but not least iron, have started to enter a field which was long dominated by precious metals such as palladium, rhodium, ruthenium, and iridium. The present review article summarizes the development of iron-, nickel-, and cobaltcatalyzed C-H functionalization reactions until the end of 2016, and discusses the scope and limitations of these transformations.

机译：由于这些金属的突出生态和经济性质，非珍贵金属催化的反应在化学上越来越重要。在金属催化的直接C-H官能化反应的子场中，近年来已经显示了越来越多的出版物，致力于本主题。镍，钴和最后但并非最不重要的是，已经开始进入一个长期以来的贵金属，例如钯，铑，钌和铱。本综述文章总结了在2016年底之前概述了铁，镍和钴催化的C-H官能化反应，并探讨了这些转变的范围和限制。

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《Chemistry: A European journal》 |2017年第39期|共27页
作者
Gerit Pototschnig; Nuno Maulide; Michael Schnerch;
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作者单位

The Warren and Katharine Schlinger Laboratory for Chemistry and Chemical Engineering Division of Chemistry and Chemical Engineering California Institute of Technology 1200 E California Blvd Pasadena California 91125 (USA);

Institute of Organic Chemistry University of Vienna W-hringerstrasse 38 1090 Vienna (Austria);

Institute of Applied Synthetic Chemistry TU Wien Getreidemarkt 9/163 1060 Vienna (Austria);

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正文语种 eng
中图分类应用化学;
关键词
base metal catalysis; C-H activation; cobalt; iron; nickel;

机译：基础金属催化;C-H激活;钴;铁;镍;

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专利

1. Direct Functionalization of C-H Bonds by Iron, Nickel, and Cobalt Catalysis [J] . Gerit Pototschnig, Nuno Maulide, Michael Schnerch Chemistry: A European journal . 2017,第39期

机译：铁，镍和钴催化的C-H键直接官能化
2. Room-Temperature C-H Bond Functionalization by Merging Cobalt and Photoredox Catalysis [J] . Kalsi Deepti, Dutta Subhradeep, Barsu Nagaraju, ACS catalysis . 2018,第9期

机译：通过合并钴和Photoredox催化来室温C-H键官能化
3. One-Pot Directing Group Formation/C-H Bond Functionalization via Copper(I) and Ruthenium(II) Catalysis [J] . Bruneau Christian, Gramage-Doria Rafael Advanced synthesis & catalysis . 2016,第23期

机译：通过铜（I）和钌（II）催化一键引导基团形成/ C-H键官能化
4. RECOVERY OF NICKEL AND COBALT DIRECTLY FROM LEACH SOLUTIONS CONTAINING IRON AND ALUMINIUM USING A NEW DSX PROCESS [C] . Wensheng Zhang, Chu Yong Cheng, Weiwei Wang ALTA Nickel-Cobalt-Copper Conference . 2016

机译：使用新的DSX工艺直接从含有铁和铝的浸出溶液中恢复镍和钴
5. Catalytic C-H Bond Functionalization by Nickel(0) N-Heterocyclic Carbene Complexes: Influence of Ligand Sterics on Selective Silylation [D] . Elsby, Matthew Ryan. 2017

机译：镍（0）N-杂环碳烯络合物的催化C-H键官能化：配体的立体异构体对选择性硅烷化的影响
6. C-H Bond Functionalization via Hydride Transfer: Direct Coupling of Unactivated Alkynes and sp3 C-H Bonds Catalyzed by Platinum Tetraiodide [O] . Paul A. Vadola, Dalibor Sames -1

机译：通过氢转移C-H键功能化：未激活炔烃的直接耦合和sp3 C-H键的催化作用白金四碘化物
7. Enantioselective nickel catalysis : exploiting activated C-H bonds [O] . Bencivenga Nicholas Ernest 2012

机译：对映选择性镍催化：利用活化的C-H键
8. Direct Selective Acylation of an Unactivated C-H Bond in a Caged Hydrocarbon.Approach to Systems for C-H Bond Functionalization That Proceed Catalytically and Selectively at High Substrate Conversion [R] . Prosser-McCartha, C. M., Hill, C. L. 1990

机译：笼型烃中未活化C-H键的直接选择性酰化。用于C-H键官能化的系统，在高基质转化下催化和选择性地进行

Direct Functionalization of C-H Bonds by Iron, Nickel, and Cobalt Catalysis

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