Two Self-Interpenetrating Copper(II)-Paddlewheel Metal-Organic Frameworks Constructed from Bifunctional Triazolate-Carboxylate Linkers

Wang Xiao-Ning; Mao Nan-Nan; Bai Yue-Ling; Zhuang Gui-Lin; Li Bao

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Two Self-Interpenetrating Copper(II)-Paddlewheel Metal-Organic Frameworks Constructed from Bifunctional Triazolate-Carboxylate Linkers

机译：两种自渗透铜（II） - 由双官能三唑酯 - 羧酸盐接头构成的覆盖金属 - 有机框架

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摘要

From the perspective of preset configuration of ligands, the introduction of triazole would be not only conducive to furnish sites rich in nitrogen, but also favorable to enhance the stability of MOF materials. Through employing two similar bifunctional triazolate carbox-ylate organic ligands, two novel self-interpenetrating copper(II)-based metal organic frameworks have been successfully constructed under solvothermal conditions, which exhibit very similar voids but different hole shapes. In addition, powder X-ray diffraction, thermogravimetry, gas sorption studies, and theoretical calculations reveal their different framework stabilities and pore environment.

机译：从配体的预设配置的角度来看，三唑的引入不仅有利于提供富含氮的遗址，还有利于提高MOF材料的稳定性。通过采用两种类似的双官能三唑甲酸羧酸盐有机配体，在溶剂热条件下成功构建了两种新的自渗铜（II）的基础金属有机骨架，其表现出非常相似的空隙但不同的孔形状。此外，粉末X射线衍射，热重试剂，气体吸附研究和理论计算揭示了它们不同的骨架稳定性和孔隙环境。

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来源
《Crystal growth & design》 |2018年第10期|共7页
作者
Wang Xiao-Ning; Mao Nan-Nan; Bai Yue-Ling; Zhuang Gui-Lin; Li Bao;
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作者单位

Huazhong Univ Sci &

Technol Sch Chem &

Chem Engn Key Lab Mat Chem Energy Convers &

Storage Wuhan 430074 Peoples R China;

Huazhong Univ Sci &

Technol Sch Chem &

Chem Engn Key Lab Mat Chem Energy Convers &

Storage Wuhan 430074 Peoples R China;

Shanghai Univ Coll Sci Drug Ctr Dept Chem Shanghai 200444 Peoples R China;

Zhejiang Univ Technol Coll Chem Engn Inst Ind Catalysis Hangzhou 310023 Zhejiang Peoples R China;

Huazhong Univ Sci &

Technol Sch Chem &

Chem Engn Key Lab Mat Chem Energy Convers &

Storage Wuhan 430074 Peoples R China;

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正文语种 eng
中图分类晶体学;
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专利

1. Two Self-Interpenetrating Copper(II)-Paddlewheel Metal-Organic Frameworks Constructed from Bifunctional Triazolate-Carboxylate Linkers [J] . Wang Xiao-Ning, Mao Nan-Nan, Bai Yue-Ling, Crystal growth & design . 2018,第10期

机译：两种自渗透铜（II） - 由双官能三唑酯 - 羧酸盐接头构成的覆盖金属 - 有机框架
2. An Unusual (6,14)-Connected Metal-Organic Framework Constructed from Two Distinct Cobalt(II) Cluster Units and a Bifunctional Organic Linker [J] . Chen Di-Ming, Tian Jia-Yue, Liu Chun-Sen Zeitschrift fur Anorganische und Allgemeine Chemie . 2016,第11a12期

机译：由两个不同的钴（II）簇单元和一个双功能有机连接基构建的异常（6,14）连接的金属有机框架
3. Defect Engineering of Copper Paddlewheel-Based Metal-Organic Frameworks of Type NOTT-100: Implementing Truncated Linkers and Its Effect on Catalytic Properties [J] . Fan Zhiying, Wang Junjun, Wang Weijia, ACS applied materials & interfaces . 2020,第34期

机译：基于铜桨轮的金属有机框架缺陷工程 - 100：实施截短的接头及其对催化性质的影响
4. Fused Hybrid Linkers for Metal-Organic Frameworks-Derived Bifunctional Oxygen Electrocatalysts [C] . Mahboob Alam, Kefeng Ping, Rohit Bhadoria, Meeting of the Electrochemical Society;International Meeting on Chemical Sensors . 2020

机译：金属有机框架衍生的双官能氧电催化剂的熔合混合动力车接头
5. Copper(II) metal-organic frameworks containing sulfonate functionalities [D] . Kulynych, Angela Dawn 2002

机译：含磺酸盐官能团的铜（II）金属-有机骨架
6. Crystal structure of polybis(μ-2-bromopyrazine)tetra-μ2-cyanido-dicopper(I)iron(II): a bimetallic metal-organic framework [O] . Olesia I. Kucheriv, Inna I. Tokmenko, Igor P. Matushko, 2018

机译：聚双（μ-2-溴吡嗪）四-μ2-氰基-二铜（I）铁（II）的晶体结构：双金属金属-有机骨架
7. Non-interpenetrated metal-organic frameworks based on copper(II) paddlewheel and oligoparaxylene-isophthalate linkers: synthesis, structure and gas adsorption [O] . Yan Yong, Juricek Michal, Coudert Francois-Xavier, 2016

机译：基于铜（II）桨轮和低聚对二甲苯-间苯二甲酸酯接头的非互穿金属有机骨架：合成，结构和气体吸附

Two Self-Interpenetrating Copper(II)-Paddlewheel Metal-Organic Frameworks Constructed from Bifunctional Triazolate-Carboxylate Linkers

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