The Coupled Chemical and Physical Dynamics Model of MALDI

Knochenmuss Richard

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The Coupled Chemical and Physical Dynamics Model of MALDI

机译：MALDI的化学和物理动力学耦合模型

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The coupled physical and chemical dynamics model of ultraviolet matrix-assisted laser desorption/ionization (MALDI) has reproduced and explained a wide variety of MALDI phenomena. The rationale behind and elements of the model are reviewed, including the photophysics, kinetics, and thermodynamics of primary and secondary reaction steps. Experimental results are compared with model predictions to illustrate the foundations of the model, coupling of ablation and ionization, differences between and commonalities of matrices, secondary charge transfer reactions, ionization in both polarities, fluence and concentration dependencies, and suppression and enhancement effects.

机译：紫外线基质辅助激光解吸/电离（MALDI）的耦合物理和化学动力学模型已经再现并解释了多种MALDI现象。审查了模型的基本原理和元素，包括一级和二级反应步骤的光物理，动力学和热力学。将实验结果与模型预测结果进行比较，以说明模型的基础，烧蚀和电离的耦合，基质之间的共性和差异，二次电荷转移反应，极性的电离，能量密度和浓度依赖性以及抑制和增强效果。

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来源
《Annual Review of Analytical Chemistry》 |2016年第null期|共40页
作者
Knochenmuss Richard;
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原文格式 PDF
正文语种 eng
中图分类物理化学计量;
关键词
coupled physical and chemical dynamics model; MALDI; ionization mechanisms; exciton pooling; ion-molecule reactions;

机译：物理化学耦合动力学模型;MALDI;电离机理;激子池;离子分子反应;

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专利

1. The Coupled Chemical and Physical Dynamics Model of MALDI [J] . Knochenmuss Richard Annual Review of Analytical Chemistry . 2016,第Null期

机译：MALDI的化学和物理动力学耦合模型
2. MALDI ionization mechanisms: The coupled photophysical and chemical dynamics model correctly predicts 'temperature'-selected spectra [J] . Knochenmuss R. Journal of mass spectrometry: JMS . 2013,第9期

机译：MALDI电离机理：耦合的光物理和化学动力学模型可以正确预测“温度”选择的光谱
3. Ion Yields in the Coupled Chemical and Physical Dynamics Model of Matrix-Assisted Laser Desorption/Ionization [J] . Knochenmuss Richard Journal of the American Society for Mass Spectrometry . 2015,第10期

机译：基质辅助激光解吸/电离的化学和物理动力学耦合模型中的离子产率
4. Coupled modelling of physical/chemical retardation and transport of CO2/CH4 for a backfilled salt rock repository [C] . H. Alkan, W. Miiller Conference on the Mechanical Behavior of Salt . 2007

机译：用于回填盐岩储存库的物理/化学延迟和CO2 / CH4的耦合建模
5. Coupled physical and biogeochemical dynamics in shallow aquatic systems: Observations, theory and models. [D] . Branco, Brett F. 2007

机译：浅水系统中的物理和生物地球化学动力学耦合：观测，理论和模型。
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7. Modeling the nitrogen fluxes in the Black Sea using a 3D coupled hydrodynamical-biogeochemical model: transport versus biogeochemical processes, exchanges across the shelf break and comparison of the shelf and deep sea ecodynamics [O] . Grégoire M., Beckers J. M. 2004

机译：使用3D耦合水动力-生物地球化学模型对黑海中的氮通量进行建模：运输与生物地球化学过程，跨架子断裂的交换以及架子与深海生态动力学的比较

The Coupled Chemical and Physical Dynamics Model of MALDI

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