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Will climate change increase ozone depletion from low-energy-electron precipitation?

机译:气候变化会增加低能电子降水造成的臭氧消耗吗?

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We investigate the effects of a strengthened stratospheric/mesospheric residual circulation on the transport of nitric oxide (NO) produced by energetic particle precipitation. During periods of high geomagnetic activity, energetic electron precipitation (EEP) is responsible for winter time ozone loss in the polar middle atmosphere between 1 and 6 hPa. However, as climate change is expected to increase the strength of the Brewer-Dobson circulation including extratropical downwelling, the enhancements of EEP NOx concentrations are expected to be transported to lower altitudes in extratropical regions, becoming more significant in the ozone budget. Changes in the mesospheric residual circulation are also considered. We use simulations with the chemistry climate model system EMAC to compare present day effects of EEP NOx with expected effects in a climate change scenario for the year 2100. In years of strong geomagnetic activity, similar to that observed in 2003, an additional polar ozone loss of up to 0.4 μmol/mol at 5 hPa is found in the Southern Hemisphere. However, this would be approximately compensated by an ozone enhancement originating from a stronger poleward transport of ozone from lower latitudes caused by a strengthened Brewer-Dobson circulation, as well as by slower photochemical ozone loss reactions in a stratosphere cooled by risen greenhouse gas concentrations. In the Northern Hemisphere the EEP NOx effect appears to lose importance due to the different nature of the climate-change induced circulation changes.
机译:我们调查了平流层/中层大气残余循环的增强对高能粒子沉淀产生的一氧化氮(NO)传输的影响。在高地磁活动期间,高能电子沉淀(EEP)导致冬季在1-6 hPa的极地中间大气中的臭氧损失。但是,由于预计气候变化会增加包括温带下流的Brewer-Dobson环流的强度,因此预计EEP NOx浓度的增加将被传送到温带地区的较低海拔,这在臭氧预算中将变得更加重要。还考虑了中层残余循环的变化。我们使用化学气候模型系统EMAC进行模拟,以比较EEP NOx的当前影响与2100年气候变化情景中的预期影响。在多年的地磁活动中,类似于2003年的观测,额外的极性臭氧损失在南半球发现在5 hPa时最高可达0.4μmol/ mol。但是,这将通过以下方式得到大致补偿:臭氧的增强,这是由于加强的Brewer-Dobson环流引起的,来自较低纬度的臭氧从极纬向的更强的向极迁移所致,以及平流层中由于温室气体浓度升高而冷却的光化学臭氧损失反应变慢。在北半球,由于气候变化引起的循环变化的不同性质,EEP NOx效应似乎失去了重要性。

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