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首页> 外文期刊>Annual Review of Physical Chemistry >Long-range resonance energy transfer in molecular systems [Review]
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Long-range resonance energy transfer in molecular systems [Review]

机译：分子系统中的远程共振能量转移[综述]

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The current state of understanding of molecular resonance energy transfer (RET) and recent developments in the field are reviewed. The development of more general theoretical approaches has uncovered some new principles underlying RET processes. This review brings many of these important new concepts together into a generalization of Forster's original theory. The conclusions of studies investigating the various approximations in Forster theory are summarized. Areas of present and future activity are discussed. The review covers Forster theory for donor-acceptor pairs and electronic coupling for singlet-singlet, triplet-triplet, and superexchange-mediated energy transfer. This includes the transition density picture of Coulombic coupling as well as electronic coupling between molecular aggregates (excitons). Spectral overlaps and ensemble energy transfer rates in disordered aggregates, the role of dielectric properties of the medium, weak versus strong coupling, and new models for energy transfer in complex molecular assemblies are also described. [References: 183]
机译：综述了对分子共振能量转移（RET）的理解现状以及该领域的最新进展。更一般的理论方法的发展发现了RET过程的一些新原理。这篇评论将许多重要的新概念整合到了Forster的原始理论中。总结了研究Forster理论中各种近似方法的研究结论。讨论了当前和将来的活动领域。这篇综述涵盖了供体-受体对的Forster理论以及单重态-单重态，三重态-三重态和超交换介导的能量转移的电子耦合。这包括库仑耦合以及分子聚集体（激子）之间电子耦合的跃迁密度图。还描述了无序聚集体中的光谱重叠和集合能量传输速率，介质介电特性的作用，弱耦合与强耦合以及复杂分子组装体中能量转移的新模型。 [参考：183]

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