Exploring alkylated ferrocene sulfonates as electrocatalysts for sulfide detection

Banks CE; Yashina AS; Tustin GJ; Lafitte VGH; Jones TGJ; Lawrence NS

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Exploring alkylated ferrocene sulfonates as electrocatalysts for sulfide detection

机译：探索烷基化二茂铁磺酸盐作为检测硫化物的电催化剂

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Alkylated ferrocene sulfonate compounds, 1,1'-dimethyl ferrocene sulfonate, t-butyl ferrocene sulfonate, ethyl ferrocene sulfonate, and n-butyl ferrocene sulfonate are explored for the electrocatalytic detection of sulfide at a boron-doped diamond electrode. Voltammetric interrogation of the ferrocene sulfonate compounds is investigated to determine oxidizing potentials, diffusion coefficients and responses towards sulfide. In the latter case, measurement of the electrocatalytic rate constants by means of chronoamperometry indicates a high electrocatalytic activity (ca. 10(3) M-1 s(-1)) towards sulfide.

机译：探索了烷基化的二茂铁磺酸盐化合物，1,1'-二甲基二茂铁磺酸盐，叔丁基二茂铁磺酸盐，乙基二茂铁磺酸盐和正丁基二茂铁磺酸盐，用于在硼掺杂金刚石电极上对硫化物进行电催化检测。研究了二茂铁磺酸盐化合物的伏安询问，以确定氧化电位，扩散系数和对硫化物的响应。在后一种情况下，通过计时电流法测量电催化速率常数表明对硫化物具有很高的电催化活性（约10（3）M-1 s（-1））。

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《Electroanalysis》 |2007年第24期|共5页
作者
Banks CE; Yashina AS; Tustin GJ; Lafitte VGH; Jones TGJ; Lawrence NS;
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正文语种 eng
中图分类电化学、电解、磁化学;
关键词
ferrocene sulfonates; hydrogen sulfide; electrocatalysis; EC'; boron-doped diamond; DOPED DIAMOND ELECTRODE; HYDROGEN-SULFIDE; GALVANIC SENSOR; OXIDATION; DERIVATIVES; ACID; FERRICYANIDE; VOLTAMMETRY; CYSTEINE; SULFUR;

机译：二茂铁磺酸盐;硫化氢;电催化;EC';掺硼金刚石;掺杂金刚石电极;氢硫化物;电化学传感器;氧化;衍生物;酸;铁氰化物;伏安;半胱氨酸;硫;

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1. Exploring alkylated ferrocene sulfonates as electrocatalysts for sulfide detection [J] . Banks CE, Yashina AS, Tustin GJ, Electroanalysis . 2007,第24期

机译：探索烷基化二茂铁磺酸盐作为检测硫化物的电催化剂
2. Amperometric detection of sulfide: An electrocatalytic reaction with ferrocene carboxylate [J] . Lawrence NS Electroanalysis . 2006,第17期

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Exploring alkylated ferrocene sulfonates as electrocatalysts for sulfide detection

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