Femtosecond laser control of intramolecular vibrations in a liquid

Nikiforov V.G.; Shmelev A.G.; Safiullin G.M.; Lobkov V.S.; Samartsev V.V.

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Femtosecond laser control of intramolecular vibrations in a liquid

机译：飞秒激光控制液体中分子内的振动

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Optical control of coherent intramolecular oscillations in chloroform CHCl3 and dimethyl sulfoxide (CH _3) _3SO is attained experimentally under normal conditions by means of femtosecond polarization spectroscopy. Nonresonant excitation of the medium is accomplished by a sequence of two linearly polarized laser pulses. The state of the medium is probed by the third pulse via the optical Kerr effect. We show that control over the vibrational dynamics of molecules on a sub-picosecond scale can be achieved by varying the delay between the excitation pulses and their relative intensity.

机译：在正常条件下，通过飞秒偏振光谱法实验性地获得了氯仿CHCl3和二甲基亚砜（CH _3）_3SO中相干分子内振荡的光学控制。介质的非共振激发是通过两个线性偏振激光脉冲序列实现的。介质的状态通过光学克尔效应由第三个脉冲探测。我们表明，可以通过改变激发脉冲及其相对强度之间的延迟来实现亚皮秒级的分子振动动力学控制。

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《Bulletin of the Russian Academy of Sciences. Physics》 |2012年第3期|共4页
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Nikiforov V.G.; Shmelev A.G.; Safiullin G.M.; Lobkov V.S.; Samartsev V.V.;
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正文语种 eng
中图分类物理学;
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1. Femtosecond laser control of intramolecular vibrations in a liquid [J] . Nikiforov V.G., Shmelev A.G., Safiullin G.M., Bulletin of the Russian Academy of Sciences. Physics . 2012,第3期

机译：飞秒激光控制液体中分子内的振动
2. Intramolecular Vibrational Dynamics in Free Polyatomic Molecules with C=O Chromophore Bond Excited by Resonant Femtosecond IR Laser Radiation [J] . Sergey V. Chekalin, Victor O. Kompanets, Pavel V. Koshlyakov, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2014,第6期

机译：飞秒红外激光辐射激发具有C = O发色团键的游离多原子分子的分子内振动动力学
3. Probing intramolecular vibrational energy re-distribution by using a pair of femtosecond-laser pulses: a theoretical model [J] . Hashimoto N., Yamanouchi K., Someda K. Chemical Physics Letters . 1998,第1a2期

机译：使用一对飞秒激光脉冲探测分子内振动能的重新分布：理论模型
4. Controlled Chemical Modification of Biomolecules by Femtosecond Laser in Polar Liquids [C] . V.E. Gruzdev, D. Korkin, B.P. Mooney, International Conference on Laser Optics . 2018

机译：飞秒激光在极性液体中对生物分子的受控化学修饰
5. Studies on Temperature Dependence of Intermolecular Vibrational Dynamics in Ionic Liquids by Femtosecond Raman-Induced Kerr Effect Spectroscopy [D] . KAKINUMA, Shohei 2019

机译：飞秒拉曼诱导克尔效应光谱研究离子液体中分子间振动动力学的温度依赖性
6. Vibration-Assisted Femtosecond Laser Drilling with Controllable Taper Angles for AMOLED Fine Metal Mask Fabrication [O] . Wonsuk Choi, Hoon Young Kim, Jin Woo Jeon, 2017

机译：具有可控锥角的振动辅助飞秒激光钻孔用于AMOLED精细金属掩模的制造
7. Vibration-Assisted Femtosecond Laser Drilling with Controllable Taper Angles for AMOLED Fine Metal Mask Fabrication [O] . Wonsuk Choi, Hoon Young Kim, Jin Woo Jeon, 2017

机译：具有可控锥角的振动辅助飞秒激光钻孔用于amOLED精细金属掩模制造
8. Intramolecular Vibrational Energy Transfer and Bond-Selected Photochemistry in Liquids [R] . Crim, F. F. 2001

机译：分子内振动能量转移和键合选择的液体光化学

Femtosecond laser control of intramolecular vibrations in a liquid

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