Complete characterization of the (D_2O)_2 ground state: High K_a rotation-tunneling levels

Frank N. Keutsch; Nir Goldman; Evgeniy N. Karyakin; Heather A. harker; Maria E. Sanz; Claude Leforestier; Richard J. Saykally

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Complete characterization of the (D_2O)_2 ground state: High K_a rotation-tunneling levels

机译：（D_2O）_2基态的完整表征：高K_a旋转隧穿能级

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We report the observation of extensive a- and c-type rotation-tunneling (RT) spectra of (D_2O)_2 for K_a = 0-4. These data allow quantification of molecular constants and tunneling splittings for a number of previously unobserved RT states of (D_2O)_2. The vibrational ground state has thus been characterized to energies as high as those of some of the intermolecular vibrations, and we present the first test of the VRT (ASP-W) potential at these high K_a states.

机译：我们报告观察到广泛的a和c型旋转隧道（RT）的（D_2O）_2的光谱K_a = 0-4。这些数据允许对许多以前未观察到的（D_2O）_2 RT状态进行分子常数定量和隧穿分裂的定量分析。因此，已将振动基态表征为具有与某些分子间振动一样高的能量，并且我们提出了在这些高K_a状态下对VRT（ASP-W）势的首次测试。

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《Faraday discussions》 |2001年第118期|共15页
作者
Frank N. Keutsch; Nir Goldman; Evgeniy N. Karyakin; Heather A. harker; Maria E. Sanz; Claude Leforestier; Richard J. Saykally;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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Complete characterization of the (D_2O)_2 ground state: High K_a rotation-tunneling levels

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