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Measurement of current-induced local heating in a single molecule junction

机译:测量单分子结中电流感应的局部加热

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We have studied the current-induced local heating effects in single molecules covalently bound to two electrodes by measuring the force required to break the molecule-electrode bonds under various conditions. The breakdown process is thermally activated, which is used to extract the effective temperature of the molecular junction as a function of applied bias voltage. We have also performed first-principles calculations of both local heating and current-induced force effects, and the results are in good agreement with the experimental findings.
机译:我们通过测量在各种条件下破坏分子-电极键所需的力,研究了电流共价键合到两个电极的单分子中的局部热效应。击穿过程是热激活的,用于提取分子结的有效温度,该温度是施加的偏置电压的函数。我们还进行了局部加热和电流感应力效应的第一性原理计算,结果与实验结果非常吻合。

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