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Enhanced probabilities of phonon-assisted optical transitions in semiconductor quantum dots

机译:半导体量子点中声子辅助光学跃迁的增强概率

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A theory of phonon-assisted optical transitions in semiconductor quantum dots is developed which takes into account the non-adiabaticity of the exciton-phonon system. The role of non-adiabaticity is shown to be of paramount importance in spherical quantum dots, where the lowest one-exciton state can be degenerat4e or quasi-degenerate. In quantum dots of lower symmetry, the effects of non-adiabaticity reveal themselves mainly due to the phonon-induced mixing of states which belong to different energy levels. Our approach is applied to explain the optical spectra of several quantum-dot structures: ensembles of spherical CdSe, CdSe_xS_(1-x) and PbS quantum dots, self-assembled InAs/GaAs and CdSe/ZnSe quantum dots, brick-shaped InAs/GaAs quantum dots and CdS/HgS/CdS quantum dot heterostructures.
机译:考虑到激子-声子系统的非绝热性,发展了一种半导体量子点中声子辅助光学跃迁的理论。非绝热的作用在球形量子点中至关重要,在球形量子点中,最低的一个激子态可以简并或简并。在较低对称性的量子点中,非绝热效应的出现主要是由于声子引起的属于不同能级的态的混合。我们的方法用于解释几种量子点结构的光谱:球形CdSe,CdSe_xS_(1-x)和PbS量子点的集合,自组装InAs / GaAs和CdSe / ZnSe量子点,砖形InAs / GaAs量子点和CdS / HgS / CdS量子点异质结构。

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