Unexpected C=N bond formation via NaI-catalyzed oxidative de-tetra-hydrogenative cross-couplings between N,N-dimethyl aniline and sulfamides

Zheng Yang; Mao Jincheng; Chen Jie; Rong Guangwei; Liu Defu; Yan Hong; Chia Yongjian; Xu Xinfang

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Unexpected C=N bond formation via NaI-catalyzed oxidative de-tetra-hydrogenative cross-couplings between N,N-dimethyl aniline and sulfamides

机译：N，N-二甲基苯胺和磺酰胺之间通过NaI催化的氧化脱四氢加氢偶合意外地形成C = N键

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A direct and convenient C=N bond formation reaction was reported, which was a de-tetra-hydrogenative cross-coupling (DTCC) reaction between N,N-dimethyl aniline and sulfamide under transition-metal-free conditions, and to give sulfonyl amidine derivatives in moderate to high yields.

机译：报道了直接和方便的C ＝ N键形成反应，其是在无过渡金属的条件下，N，N-二甲基苯胺与磺酰胺之间的脱四氢交叉偶联（DTCC）反应，并得到磺酰基am中高收益的衍生产品。

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来源
《RSC Advances》 |2015年第62期|共5页
作者
Zheng Yang; Mao Jincheng; Chen Jie; Rong Guangwei; Liu Defu; Yan Hong; Chia Yongjian; Xu Xinfang;
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正文语种 eng
中图分类化学;
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1. Unexpected C=N bond formation via NaI-catalyzed oxidative de-tetra-hydrogenative cross-couplings between N,N-dimethyl aniline and sulfamides [J] . Zheng Yang, Mao Jincheng, Chen Jie, RSC Advances . 2015,第62期

机译：N，N-二甲基苯胺和磺酰胺之间通过NaI催化的氧化脱四氢加氢偶合意外地形成C = N键
2. Synthesis and characterization of some new aromatic diamine monomers from oxidative coupling of anilines and substituted aniline with 4-amino-N,N-dimethyl aniline [J] . Kuestan A. Ibrahim Arabian journal of chemistry . 2014,第6期

机译：苯胺和取代苯胺与4-氨基-N，N-二甲基苯胺的氧化偶联合成某些新型芳族二胺单体
3. Palladium(II)-Catalyzed Dehydrogenative Cross-Coupling between Two C_(sp~3)-H Bonds: Unexpected C=C Bond Formation [J] . Gaocan Li, Shengyou Qian, Chunxia Wang Angewandte Chemie . 2013,第30期

机译：两个C_（sp〜3）-H键之间钯（II）催化的脱氢交叉偶联：意外的C = C键形成
4. Effect of Benzoyl peroxide/N, N-dimethyl aniline initiating system on material removal rate in abrasive-free polishing of hard disk substrate [C] . Ting Jiang, Hong Lei International Conference on Planarization/CMP Technology . 2014

机译：过氧化苯甲酰/ N，N-二甲基苯胺引发体系对硬盘基板无磨料抛光中材料去除率的影响
5. Carbon-Carbon Bond Formation and Unexpected Carbon-Hydrogen Bond Activation at Adjacent Metal Centres. [D] . MacDougall, Tiffany Jayne. 2012

机译：相邻金属中心的碳-碳键形成和意外的碳-氢键活化。
6. Oxidative Palladium(II) Catalysis: A Highly Efficient and Chemoselective Cross-Coupling Method for Carbon-Carbon Bond Formation under Base-Free and Nitrogenous-Ligand Conditions [O] . Kyung Soo Yoo, Cheol Hwan Yoon, Kyung Woon Jung -1

机译：氧化钯（II）催化：在无碱和氮配体条件下形成碳-碳键的高效且化学选择性的交叉偶联方法
7. Synthesis and characterization of some new aromatic diamine monomers from oxidative coupling of anilines and substituted aniline with 4-amino-N,N-dimethyl aniline [O] . Kuestan A. Ibrahim 2014

机译：苯胺与取代苯胺与4-氨基-N，N-二甲基苯胺氧化偶联的新型芳香二胺单体的合成与表征
8. Algal-Induced Decay and Formation of Hydrogen Peroxide in Water: Its Possible Role in Oxidation of Anilines by Algae [R] . Zepp, R. G. , Skurlatov, Y. I. , Pierce, J. T. 1986

机译：藻类诱导的腐烂和水中过氧化氢的形成：藻类氧化苯胺的可能作用

Unexpected C=N bond formation via NaI-catalyzed oxidative de-tetra-hydrogenative cross-couplings between N,N-dimethyl aniline and sulfamides

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