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Neutron scattering analysis of low-frequency modes in silica

机译:二氧化硅中低频模式的中子散射分析

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We report coherent inelastic neutron scattering results in vitreous silica at temperatures up to 1673 K, 200 K above the glass transition. As in earlier low-temperature data, clear evidence is seen for non-sound-wave modes at the boson peak. Contrary to other glass formers, silica shows nearly no fast relaxations at the glass transition. The combination of the neutron spectra with recent X-ray Brillouin data allows the identification of the scattering mechanisms for high-frequency sound waves in the glass. Below 1 THz, one has resonant scattering from low-frequency vibrations and above 1 THz, Rayleigh scattering from the atomic disorder. [References: 30]
机译:我们报告相干的非弹性中子散射结果,在高达1673 K(比玻璃化转变温度高200 K)的温度下,玻璃状二氧化硅。与早期的低温数据一样,在玻色子峰处也可以看到明显的非声波模式证据。与其他玻璃形成剂相反,二氧化硅在玻璃化转变时几乎没有快速松弛。将中子光谱与最新的X射线布里渊数据相结合,可以确定玻璃中高频声波的散射机制。低于1 THz时,低频振动产生共振散射,高于1 THz时,原子混乱引起瑞利散射。 [参考:30]

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