Intramolecular Dipolar Cycloaddition Reactions of Azomethine Ylides

lain Coldham; Richard Hufton

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Intramolecular Dipolar Cycloaddition Reactions of Azomethine Ylides

机译：甲亚胺叶立德分子的分子内偶极环加成反应

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It was in 1963 that Huisgen laid out the classification of 1,3-dipoles and the concepts for 1,3-dipolar cycloaddition reactions,although it was not until 1976 that the first intramolecular 1,3-dipolar cycloaddition reaction of an azomethine ylide was reported.Since then,impressive developments have been described in this area,with the establishment of various useful methods for the formation of azomethine ylides and the determination of the requirements for a successful intramolecular cycloaddition reaction.Use of this methodology for the synthesis of pyrrolidine-and pyrrole-containing natural products has been expanding rapidly.This review aims to describe the background and mechanisms of azomethine ylide formation and intramolecular cycloaddition,giving a critical account including the

机译：1963年，Huisgen提出了1,3-偶极的分类和1,3-偶极环加成反应的概念，尽管直到1976年才出现了第一个分子内偶氮甲meth基内酯的1,3-偶极环加成反应。从那时起，该领域的发展得到了令人瞩目的发展，建立了各种有用的方法来形成偶氮甲亚胺，并确定了成功的分子内环加成反应的要求。该方法用于吡咯烷-的合成本综述旨在描述偶氮次甲基叶立德形成和分子内环加成反应的背景和机理，并给出了包括

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《Chemical Reviews》 |2005年第7期|共45页
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lain Coldham; Richard Hufton;
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1. Intramolecular Dipolar Cycloaddition Reactions of Azomethine Ylides [J] . lain Coldham, Richard Hufton Chemical Reviews . 2005,第7期

机译：甲亚胺叶立德分子的分子内偶极环加成反应
2. Auxiliary-Controlled Asymmetric [3+2]-Dipolar Cycloaddition of Azomethine Ylides Generated from Au-Catalyzed Intramolecular Redox Reaction of Nitronyl Alkynes [J] . Jaewon Jeong, Hyun-Suk Yeom, Ohyun Kwon, Chemistry, an Asian journal . 2011,第8期

机译：辅助控制的不对称[3 + 2]-偶极环加成反应的偶氮亚基叶立德从Au催化的硝酰基炔烃分子内氧化还原反应中生成。
3. [3+2]-cycloaddition of nonstabilized azomethine ylides, part 9: A general approach for the construction of X-azabicyclo[m.2.1]alkanes optically pure form by asymmetric 1,3-dipolar cycloaddition reactions [J] . Pandey G., Mohanakrishnan AK., Laha JK. Tetrahedron letters: The International Journal for the Rapid Publication of Preliminary Communications in Organic Chemistry . 1999,第33期

机译：[3 + 2]-环加成的不稳定的甲亚胺基亚胺，第9部分：通过不对称1,3-偶极环加成反应构建光学纯形式的X-氮杂双环[m.2.1]烷烃的一般方法
4. A facial regioselective synthesis of novel pyrrolizidines through azomethine ylide cycloaddition reaction [C] . Yaghoub Sarrafi, Kamal Alimohammadi European Symposium on Organic Chemistry . 2009

机译：通过氮杂甲酸钠环加入反应进行新型吡咯烷的面部区域选择性合成
5. 1,3-Dipolar cycloaddition of azomethine ylides to carbon(60) and carbon(70): Combinatorial synthesis of a small library of pyridazines using polymer-bound azodicarboxylate resin. [D] . Tan, Xuefei. 2002

机译：1,3-偶极亚甲基环向碳（60）和碳（70）的偶极环加成反应：使用聚合物结合的偶氮二羧酸酯树脂组合合成一个小的哒嗪类文库。
6. A Novel One-Pot Green Synthesis of Dispirooxindolo-pyrrolidines via13-Dipolar Cycloaddition Reactions of Azomethine Ylides [O] . Abdulrahman I. Almansour, Natarajan Arumugam, Raju Suresh Kumar, 2015

机译：通过偶氮甲Y叶立德的13-偶极环加成反应合成新颖的一锅绿色双螺并吡咯并吡咯烷类化合物
7. Synthesis of Chromen[4,3-b]pyrrolidines by Intramolecular 1,3-Dipolar Cycloadditions of Azomethine Ylides: An Experimental and Computational Assessment of the Origin of Stereocontrol [O] . Costa, Paulo R.R., Sansano, Jose M., Cossío, Unai, 2015

机译：分子内的1，3-偶极环甲亚胺叶立德加成反应合成Chromen [4,3-b]吡咯烷：立体控制起源的实验和计算评估

Intramolecular Dipolar Cycloaddition Reactions of Azomethine Ylides

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