Symmetrical and unsymmetrical dizinc complexes as models for the active sites of hydrolytic enzymes

Jarenmark M; Kappen S; Haukka M; Nordlander E

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Symmetrical and unsymmetrical dizinc complexes as models for the active sites of hydrolytic enzymes

机译：对称和不对称二锌配合物作为水解酶活性位点的模型

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摘要

Dinuclear carboxylate-bridged zinc complexes of one symmetric and one asymmetric phenolate-based ligand catalyse the transesterification of 2-hydroxypropyl-p-nitrophenyl phosphate (HPNP) at different rates, with an unsymmetrical complex being more active than a symmetric one.

机译：一种对称和一种基于不对称酚盐的配体的双核羧酸盐桥联的锌络合物以不同的速率催化2-羟丙基-对硝基苯基磷酸酯（HPNP）的酯交换反应，其中不对称的络合物比对称的络合物更具活性。

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《Dalton transactions: An international journal of inorganic chemistry》 |2008年第8期|共4页
作者
Jarenmark M; Kappen S; Haukka M; Nordlander E;
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正文语种 eng
中图分类化学;
关键词
PURPLE ACID-PHOSPHATASES; METHANE MONOOXYGENASE; ZINC(II) COMPLEXES; CRYSTAL-STRUCTURE; NICKEL-COMPLEXES; DINUCLEAR; ZINC(II)-IRON(III); PHOSPHOTRIESTERASE; BINUCLEAR; LIGANDS;

机译：紫色磷酸;甲醇单加氧酶;锌（II）络合物;晶体结构;镍络合物;膳食;锌（II）-铁（III）;磷酸酯酶;双核糖;脂质;

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1. Symmetrical and unsymmetrical dizinc complexes as models for the active sites of hydrolytic enzymes [J] . Jarenmark M, Kappen S, Haukka M, Dalton transactions: An international journal of inorganic chemistry . 2008,第8期

机译：对称和不对称二锌配合物作为水解酶活性位点的模型
2. Unsymmetrical dizinc complexes as models for the active sites of phosphohydrolases [J] . Jarenmark M., Csapó E., Singh J., Dalton transactions: An international journal of inorganic chemistry . 2010,第35期

机译：非对称二锌配合物作为磷酸水解酶活性位点的模型
3. Modeling the Active Site of the Purple Acid Phosphatase Enzyme with Hetero-Dinuclear Mixed Valence M(II)–Fe(III) [M = Zn, Ni, Co, and Cu] Complexes Supported over a [N₆O] Unsymmetrical Ligand [J] . Chandni Pathak, Sandeep K. Gupta, Manoj Kumar Gangwar, ACS Omega . 2017,第8期

机译：用杂酸磷酸酶与杂核混合价M（II）-Fe（III）[M = Zn，Ni，Co，Co和Cu]复合物在[n _{6 O]非对称配体}
4. A Multi-scale Modeling Study of MDH-Catalyzed Methanol Oxidation: The Effect of the Ion in the Enzyme Active Site [C] . Purnima Kharidehal, Daniela S. Mainardi AIChE annual meeting . 2011

机译：MDH催化甲醇氧化的多尺度建模研究：离子在酶活性位点的影响
5. Model complexes as probes of heme and nonheme enzymatic mechanisms: (1) Ferric peroxo porphyrin complexes as mimics of P450 enzymes using the ferric peroxo species as an active oxidant. (2) Strongly oxidizing iron (III) complexes as models of the active site intermediates of lipoxygenase. [D] . Wertz, Diana L. 1999

机译：将复合物建模为血红素和非血红素酶机制的探针：（1）使用过氧化铁物种作为活性氧化剂，将过氧化铁卟啉复合物模拟为P450酶。（2）强氧化铁（III）络合物作为脂氧合酶活性位点中间体的模型。
6. Models for Unsymmetrical Active Sites in Metalloproteins: Structural Redox and Magnetic Properties of Bimetallic Complexes with MII–(μ-OH)–FeIII Cores [O] . Yohei Sano, Nathanael Lau, Andrew C. Weitz, -1

机译：金属蛋白中不对称活性位点的模型：具有MII–（μ-OH）–FeIII核的双金属配合物的结构氧化还原和磁性
7. Modeling the Active Site of the Purple Acid Phosphatase Enzyme with Hetero-Dinuclear Mixed Valence M(II)–Fe(III) [M = Zn, Ni, Co, and Cu] Complexes Supported over a [N6O] Unsymmetrical Ligand [O] . Chandni Pathak, Sandeep K. Gupta, Manoj Kumar Gangwar, 2017

机译：用[N6O]不对称配体负载的异双核混合价m（II）-Fe（III）[m = Zn，Ni，Co和Cu]配合物模拟紫色酸性磷酸酶活性位点

Symmetrical and unsymmetrical dizinc complexes as models for the active sites of hydrolytic enzymes

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