NATURAL PRODUCT INSPIRED meta/para'-BIARYL ETHER LACTAM MACROCYCLES BY DOUBLE UGIMULTICOMPONENT REACTIONS

Bernhard Westermann; Dirk Michalik; Angela Schaks

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NATURAL PRODUCT INSPIRED meta/para'-BIARYL ETHER LACTAM MACROCYCLES BY DOUBLE UGIMULTICOMPONENT REACTIONS

机译：通过双UGI多组分反应激发天然产物的间/对'-双'-醚内酰胺微环

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Isonitrile meta/para'-functionalized biaryl ethers can serve as key building blocks for the highly efficient and diverse one step production of natural product inspired peptide/peptoid macrocycles,thereby forming up to 54-membered rings with eight or even sixteen new bonds.Aliphatic diamine and diacid tethers give access to two different classes of biaryl ether cyclopeptoids,either with exo/endo or exclusively endo dipeptidic moieties.

机译：异腈的meta / para'-官能化的芳基醚可以作为高效方法和关键步骤，一步一步生产天然产物启发的肽/类肽大环化合物，从而形成多达54个成员的具有8个或什至16个新键的环。二胺和二酸系链可通过exo / endo或仅具有内二肽部分访问两种不同类型的联芳醚环类肽。

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《Heterocycles: An International Journal for Reviews and Communications in Heterocyclic Chemistry》 |2007年第1期|共10页
作者
Bernhard Westermann; Dirk Michalik; Angela Schaks;
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中图分类杂环化合物;
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1. NATURAL PRODUCT INSPIRED meta/para'-BIARYL ETHER LACTAM MACROCYCLES BY DOUBLE UGIMULTICOMPONENT REACTIONS [J] . Bernhard Westermann, Dirk Michalik, Angela Schaks Heterocycles: An International Journal for Reviews and Communications in Heterocyclic Chemistry . 2007,第1期

机译：通过双UGI多组分反应激发天然产物的间/对'-双'-醚内酰胺微环
2. Rapid and diverse route to natural product-like biaryl ether containing macrocycles [Review] [J] . Cristau P., Vors JP., Zhu JP. Tetrahedron . 2003,第40期

机译：快速且多样化的途径获得含有大环化合物的天然产物状联芳醚[综述]
3. Efficient synthesis of substituted styrenes and biaryls (or heteroaryls) with regioselective reactions of ortho -, meta -, and para-bromobenzyl bromide [J] . AnselmiE., AbarbriM., DuchêneA., Synthesis: International Journal of Methods in Synthetic Organic Chemistry . 2012,第13期

机译：有效合成邻位，间位和对溴苄基溴的区域选择性反应的取代苯乙烯和联芳基（或杂芳基）
4. Synthesis of Biologically Relevant Natural and Unnatural Gamraα-Lactones and Lactams via Tandem Allylboration/Cyclization Reactions [C] . Tim G. Elford, Dennis G. Hall European Symposium on Organic Chemistry . 2009

机译：通过串联烯丙基硼酸盐/环化反应合成生物相关天然和非自然GAMRAα-内酯和内酰胺的方法
5. Development of chiral 1,5-diaza-cis-decalin ligands for asymmetric syntheses, Enantioselective oxidative biaryl coupling reactions, [and] Synthetic studies toward perylenequinone natural products. [D] . Li, Xiaolin. 2002

机译：开发用于不对称合成的手性1,5-二氮杂-顺式十氢化萘配体，对映选择性氧化性联芳偶合反应，以及对and醌天然产物的合成研究。
6. Discussion Addendum for: 4-Methoxy-4-nitrophenyl. Recent Advances in the Stille Biaryl Coupling Reaction and Applications in Complex Natural Products Synthesis [O] . Robert M. Williams, J. Stille, A. Echavarren, -1

机译：讨论的附录：4-甲氧基-4-硝基苯。在施蒂尔二芳基偶联反应的研究进展并在复杂的天然产物合成中的应用
7. Secondary Products from Intramolecular Cycloadditions of Azidoalkyl Enol Ethers and Azidoalkyl Vinyl Bromides: 1-Azadienes, Their Reactions with Diphenylketene, and Radical Cyclizations To Form Bi- and Tricyclic Lactams [O] . John T. R. Liddon, Peter J. Lindsay-Scott, Jeremy Robertson 2019

机译：二氮烷基烯醇醚和氮杂烷基乙烯基溴化物的分子内环加成的二次产物：1-己二烯，其与二苯基酮的反应，以及形成双和三环内酰胺的自由基环化
8. Rates and Mechanisms of Complexation Reactions of Cations with Crown Ethers and Related Macrocycles [R] . Eyring, E. M., Petrucci, S. 1989

机译：阳离子与冠醚和相关大环化合物络合反应的速率和机理

NATURAL PRODUCT INSPIRED meta/para'-BIARYL ETHER LACTAM MACROCYCLES BY DOUBLE UGIMULTICOMPONENT REACTIONS

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