Novel Peptide Chemistry in Terrestrial Animals: Natural Luciferin Analogues from the Bioluminescent Earthworm Fridericia heliota

Dubinnyi Maxim A.; Tsarkova Aleksandra S.; Petushkov Valentin N.; Kaskova Zinaida M.; Rodionova Natalja S.; Kovalchuk Sergey I.; Ziganshin Rustam H.; Baranov Mikhail S.; Mineev Konstantin S.; Yampolsky Ilia V.

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Novel Peptide Chemistry in Terrestrial Animals: Natural Luciferin Analogues from the Bioluminescent Earthworm Fridericia heliota

机译：陆生动物中的新型肽化学：来自生物发光Earth Fridericia heliota的天然萤光素类似物

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We report isolation and structure elucidation of AsLn5, AsLn7, AsLn11 and AsLn12: novel luciferin analogs from the bioluminescent earthworm Fridericia heliota. They were found to be highly unusual modified peptides, comprising either of the two tyrosine-derived chromophores, CompX or CompY and a set of amino acids, including threonine, gamma-aminobutyric acid, homoarginine, and unsymmetrical N,N-dimethylarginine. These natural compounds represent a unique peptide chemistry found in terrestrial animals and rise novel questions concerning their biosynthetic origin.

机译：我们报告了AsLn5，AsLn7，AsLn11和AsLn12的分离和结构解析：来自生物发光earthFridericia heliota的新型荧光素类似物。发现它们是高度不寻常的修饰肽，包含两个酪氨酸衍生的发色团CompX或CompY和一组氨基酸，包括苏氨酸，γ-氨基丁酸，高精氨酸和不对称的N，N-二甲基精氨酸。这些天然化合物代表了在陆生动物中发现的独特肽化学，并提出了有关其生物合成来源的新问题。

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《Chemistry: A European journal》 |2015年第10期|共6页
作者
Dubinnyi Maxim A.; Tsarkova Aleksandra S.; Petushkov Valentin N.; Kaskova Zinaida M.; Rodionova Natalja S.; Kovalchuk Sergey I.; Ziganshin Rustam H.; Baranov Mikhail S.; Mineev Konstantin S.; Yampolsky Ilia V.;
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正文语种 eng
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bioluminescence; Fridericia heliota; luciferin; peptides; structure elucidation;

机译：生物发光;日光参;萤光素;肽;结构解析;

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1. Novel Peptide Chemistry in Terrestrial Animals: Natural Luciferin Analogues from the Bioluminescent Earthworm Fridericia heliota [J] . Dubinnyi Maxim A., Tsarkova Aleksandra S., Petushkov Valentin N., Chemistry: A European journal . 2015,第10期

机译：陆生动物中的新型肽化学：来自生物发光Earth Fridericia heliota的天然萤光素类似物
2. CompX, a luciferin-related tyrosine derivative from the bioluminescent earthworm Fridericia heliota. Structure elucidation and total synthesis [J] . Valentin N. Petushkov, Aleksandra S. Tsarkova, Maxim A. Dubinnyi Tetrahedron letters: The International Journal for the Rapid Publication of Preliminary Communications in Organic Chemistry . 2014,第2期

机译：CompX，来自生物发光earth Fridericia heliota的萤光素相关酪氨酸衍生物。结构阐明和全合成
3. LC-MS and microscale NMR analysis of luciferin-related compounds from the bioluminescent earthworm Fridericia heliota [J] . Simone M. Marques, Valentin N. Petushkov Laboratory of Photobiology Institute of Biophysics Siberian Branch of the Russian Academy of Sciences Akademgorodok 660036 Krasnoyarsk Russia, Natalja S. Rodionova Journal of Photochemistry and Photobiology, B. Biology: Official Journal of the European Society for Photobiology . 2011,第3期

机译：生物发光earthFridericia heliota的萤光素相关化合物的LC-MS和微型NMR分析
4. Synthesis of several substituted at position 3 analogues of the naturally occurring peptide Tyr-MIF-1 (Tyr-Pro-Leu-Gly-NH_2) [C] . Svetlana S.Pancheva, Rositca J.Hristova, Efrossina P.Popgeorgieva, European Peptide Symposium . 2002

机译：在天然存在的肽Tyr-MIF-1的第3位类似物中的合成替代（Tyr-Pro-Leu-Gly-NH_2）
5. Chemical Synthesis and Biological Evaluation of Naturally Occurring Cyclic Peptides and their Analogues: Lacticin 3147 A2 and Neopetrosiamides [D] . Liu, Hongqiang 2010

机译：天然存在的环状肽及其类似物的化学合成，生物学评估：Lacticin 3147 A2和新石油酰胺
6. A Biocompatible Split Luciferin Reaction and its Application for Non-Invasive Bioluminescent Imaging of Protease Activity in Living Animals [O] . Aurélien Godinat, Ghyslain Budin, Alma R. Molares, -1

机译：生物相容性分裂萤光素反应及其在动物体内蛋白酶活性非侵入性生物发光成像中的应用
7. D-Luciferin, derivatives and analogues: synthesis and in vitro/in vivo luciferase-catalyzed bioluminescent activity [O] . Giuseppe Meroni, Mehdi Rajabi, Enzo Santaniello 2009

机译：D-荧光素，衍生物和类似物：合成和体外/体内荧光素酶催化的生物发光活性

Novel Peptide Chemistry in Terrestrial Animals: Natural Luciferin Analogues from the Bioluminescent Earthworm Fridericia heliota

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