Natural heterogeneous catalysis with immobilised oxidase biocatalysts

Mattey Ashley P.; Sangster Jack J.; Ramsden Jeremy I; Baldwin Christopher; Birmingham William R.; Heath Rachel S.; Angelastro Antonio; Turner Nicholas J.; Cosgrove Sebastian C.; Flitsch Sabine L.

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Natural heterogeneous catalysis with immobilised oxidase biocatalysts

机译：固定化氧化酶生物催化剂的天然异质催化

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The generation of immobilised oxidase biocatalysts allowing multifunctional oxidation of valuable chemicals using molecular oxygen is described. Engineered galactose oxidase (GOase) variants M-1 and M3-5, an engineered choline oxidase (AcCO6) and monoamine oxidase (MAO-N D9) displayed long-term stability and reusability over several weeks when covalently attached on a solid support, outperforming their free counterparts in terms of stability (more than 20 fold), resistance to heat at 60 degrees C, and tolerance to neat organic solvents such as hexane and toluene. These robust heterogenous oxidation catalysts can be recovered after each reaction and be reused multiple times for the oxidation of different substrates.

机译：描述了使用分子氧的允许多功能氧化有价值的化学品的固定化氧化酶生物催化剂的产生。工程半乳糖氧化酶（GOASE）变体M-1和M3-5，工程胆碱氧化酶（ACCO6）和单胺氧化酶（MAO-N D9）在固体载体上共价附着时显示长期稳定性和可重用性，优于固体载体，表现优于在稳定性（超过20倍）的自由对应物，60℃的耐热性，以及纯与己烷和甲苯的耐种有机溶剂的耐受性。可以在每次反应后回收这些稳健的异源氧化催化剂，并在多次重复使用以氧化不同底物。

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《RSC Advances》 |2020年第33期|共5页
作者
Mattey Ashley P.; Sangster Jack J.; Ramsden Jeremy I; Baldwin Christopher; Birmingham William R.; Heath Rachel S.; Angelastro Antonio; Turner Nicholas J.; Cosgrove Sebastian C.; Flitsch Sabine L.;
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Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

Univ Manchester Manchester Inst Biotechnol Dept Chem 131 Princess St Manchester M1 7DN Lancs England;

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正文语种 eng
中图分类化学;
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1. Natural heterogeneous catalysis with immobilised oxidase biocatalysts [J] . Mattey Ashley P., Sangster Jack J., Ramsden Jeremy I, RSC Advances . 2020,第33期

机译：固定化氧化酶生物催化剂的天然异质催化
2. Catalysis with gold complexes immobilised on carbon nanotubes by π-π Stacking interactions: Heterogeneous catalysis versus the boomerang effect [J] . Vriamont C., Devillers M., Riant O., Chemistry: A European journal . 2013,第36期

机译：通过π-π堆积相互作用固定在碳纳米管上的金络合物的催化作用：多相催化与回旋镖效应
3. Immobilised whole-cell recombinant monoamine oxidase biocatalysis [J] . Zajkoska Petra, Rosenberg Michal, Heath Rachel, Applied Microbiology and Biotechnology . 2015,第3期

机译：固定化全细胞重组单胺氧化酶的生物催化
4. An optical glucose biosensor based on derfived glucose oxidase immobilised onto a sol-gel matrix [C] . S de Marcos, J.Galindo, JF Sierra, European conference on solid-state transducers;UK conference on sensors and their applications . 1998

机译：基于固定的葡萄糖氧化酶的光学葡萄糖生物传感器，固定在溶胶-凝胶基质上
5. Solid phase biocatalysis of natural products in aqueous and non-aqueous media: Biocatalyst development and reaction strategies. [D] . Akbar, Umar. 2007

机译：在水性和非水性介质中天然产物的固相生物催化：生物催化剂的开发和反应策略。
6. Sol-Gel Immobilisation of Lipases: Towards Active and Stable Biocatalysts for the Esterification of Valeric Acid [O] . Soledad Cebrián-García, Alina M. Balu, Araceli García, 2018

机译：脂肪酶的溶胶-凝胶固定化：朝着稳定和稳定的戊酸酯化生物催化剂的方向发展。
7. Natural Heterogeneous Catalysis with Immobilised Oxidase Biocatalysts [O] . Ashley P. Mattey, Jack J. sangster, Christopher Baldwin, 2020

机译：固定化氧化酶生物催化剂的天然异质催化

Natural heterogeneous catalysis with immobilised oxidase biocatalysts

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