Guest encapsulations in non- porous crystals of fully fluorinated dinuclear metal complexes with the M2O2 core (M=Fe3+, Co2+, Ni2+)

Gonda Ryu; Rzeznicka Izabela I.; Kinoshita Yuki; Uchida Sayaka; Hori Akiko

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Guest encapsulations in non- porous crystals of fully fluorinated dinuclear metal complexes with the M2O2 core (M=Fe3+, Co2+, Ni2+)

机译：使用M2O2核心的完全氟化的二核金属配合物的非多孔晶体中的客体封装（M = Fe3 +，CO2 +，Ni2 +）

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Two different coordination types of fully fluorinated dinuclear metal complexes, [Fe2L4(OMe)(2)] and [M2L4(OH2)(2)] (M = Co2+, Ni2+ and HL = bis(pentafluorobenzoyl)methane), were obtained. All of the complexes form non-porous crystals, which act as hosts for the adsorption of various benzene derivatives, e.g., benzene, toluene, p-xylene, anisole, and small gas molecules, e.g., CO2, O-2, and NO. The complex of iron selectively adsorbs NO in high amounts and the complex of cobalt is found to store adsorbed O-2.

机译：得到两种不同的配位类型的完全氟化的二核金属配合物，得到[Fe2L4（OME）（2）]和[M2L4（OH 2）]和[M2L4（OH2）]（M = CO 2 +，Ni2 +和HL = BIS（五氟苯甲酰基）甲烷）。所有复合物形成无多孔晶体，其作为吸附各种苯衍生物的宿主，例如苯，甲苯，对二甲苯，苯甲醚和小气体分子，例如CO 2，O-2和NO。铁的复合物在大量中选择性地吸附不含钴的复合物，以存储吸附的O-2。

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来源
《Dalton transactions: An international journal of inorganic chemistry》 |2019年第25期|共5页
作者
Gonda Ryu; Rzeznicka Izabela I.; Kinoshita Yuki; Uchida Sayaka; Hori Akiko;
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作者单位

Shibaura Inst Technol Grad Sch Sci &

Engn Minuma ku Fukasaku 307 Saitama 3378570 Japan;

Shibaura Inst Technol Grad Sch Sci &

Engn Minuma ku Fukasaku 307 Saitama 3378570 Japan;

Univ Tokyo Sch Arts &

Sci Dept Basic Sci Meguro Ku 3-8-1 Komaba Tokyo 1538902 Japan;

Univ Tokyo Sch Arts &

Sci Dept Basic Sci Meguro Ku 3-8-1 Komaba Tokyo 1538902 Japan;

Shibaura Inst Technol Grad Sch Sci &

Engn Minuma ku Fukasaku 307 Saitama 3378570 Japan;

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正文语种 eng
中图分类化学;无机化学;
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1. Guest encapsulations in non- porous crystals of fully fluorinated dinuclear metal complexes with the M2O2 core (M=Fe3+, Co2+, Ni2+) [J] . Gonda Ryu, Rzeznicka Izabela I., Kinoshita Yuki, Dalton transactions: An international journal of inorganic chemistry . 2019,第25期

机译：使用M2O2核心的完全氟化的二核金属配合物的非多孔晶体中的客体封装（M = Fe3 +，CO2 +，Ni2 +）
2. Synthesis, single crystal X-ray, spectroscopic characterization and biological activities of Mn2+, Co2+, Ni2+ and Fe3+ complexes [J] . Journal of Molecular Structure . 2020,第期

机译：Mn2 +，CO2 +，Ni2 +和Fe3 +复合物的合成，单晶X射线，光谱表征和生物活性
3. Analysis of metal ion-induced DNA damage, apoptosis, and necrosis in human (Jurkat) T-cells demonstrates Ni2+ and V3+ are more toxic than other metals: Al3+, Be2+, Co2+, Cr3+, Cu2+, Fe3+, Mo5+, Nb5+, Zr2+. [J] . Caicedo M, Jacobs JJ, Reddy A, Journal of biomedical materials research, Part A . 2008,第4期

机译：金属离子诱导的人类T细胞（Jurkat）的DNA损伤，凋亡和坏死的分析表明，Ni2 +和V3 +的毒性比其他金属更高：Al3 +，Be2 +，Co2 +，Cr3 +，Cu2 +，Fe3 +，Mo5 +，Nb5 +，Zr2 +。
4. Micro-Columnar Crystals with (-O=V-Pd-)_n Infinite Chain Structures Assembled by Hetero-Dinuclear Metal Complexes [C] . Y. Funahashi, T. Kamimura, M. Mizutani, Asian International Conference on Advanced Materials . 2006

机译：具有（-O = V-PD - ）_ n无限链结构的微柱状晶体（-O = V-PD - ）杂交链结构
5. Raman spectroscopy of DNA-metal complexes. II. The thermal denaturation of DNA in the presence of Sr2+ Ba2+ Mg2+ Ca2+ Mn2+ Co2+ Ni2+ and Cd2+. [O] . J G Duguid, V A Bloomfield, J M Benevides, 1995

机译：DNA-金属配合物的拉曼光谱。二。在Sr2 +Ba2 +Mg2 +Ca2 +Mn2 +Co2 +Ni2 +和Cd2 +的存在下DNA的热变性。
6. Synthesis, characterization and bioactivity ¬¬¬¬Zn2+, Cu2+, Ni2+, Co2+, Mn2+, Fe3+, Ru3+, VO2+ and UO22+ complexes of 2-hydroxy-5-((4-nitrophenyl)diazenyl)benzylidene)-2-(p-tolyl- amino)acetohydrazide [O] . M. M. E. Shakdofa, A. N. Al-Hakimi, F. A. Elsaied, 2017

机译：合成，表征和生物活性¬Zn2+，Cu2 +，Ni2 +，Co2 +，mn2 +，Fe3 +，Ru3 +，VO2 +和UO22 + 2-羟基-5 - （（4-硝基苯基）二氮烯基）亚苄基）-2-（p-的配合物）甲苯基 - 氨基）乙酰肼

Guest encapsulations in non- porous crystals of fully fluorinated dinuclear metal complexes with the M2O2 core (M=Fe3+, Co2+, Ni2+)

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