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首页> 外文期刊>Geochemistry, geophysics, geosystems >In Situ Quantitative Raman Detection of Dissolved Carbon Dioxide and Sulfate in Deep‐Sea High‐Temperature Hydrothermal Vent Fluids
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In Situ Quantitative Raman Detection of Dissolved Carbon Dioxide and Sulfate in Deep‐Sea High‐Temperature Hydrothermal Vent Fluids

机译：原位定量拉曼检测溶解二氧化碳和深海高温热水通气流体中的硫酸盐

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Abstract > Carbon dioxide emitted from hydrothermal vents, as an important part of the global carbon cycle, can directly affect hydrothermal ecosystems. However, traditional chemical analysis methods cannot directly measure the concentrations of dissolved CO <sub>2</sub> in high‐temperature hydrothermal fluids. Although in situ mass spectrometry has been applied to the measurements of deep sea, it cannot be used to detect high‐temperature fluids. In this study, an in situ Raman quantitative method for measuring dissolved CO <sub>2</sub> suitable for a hydrothermal environment is established. The Raman relative intensity of CO <sub>2</sub> displayed a linear relationship with increasing concentration of CO <sub>2</sub> under the investigated conditions (up to 300°C and 40 MPa), allowing this in situ measurement method to be applied to most hydrothermal fields worldwide. Moreover, we find that the quantitative calibration curve for <mat:math display="inline" altimg="urn:x-wiley:15252027:media:ggge21587:ggge21587-math-0003" wiley:location="equation/ggge21587-math-0003.png"> <mat:msubsup> <mat:mrow> <mat:mtext>SO</mat:mtext> </mat:mrow> <mat:mrow> <mat:mn>4</mat:mn> </mat:mrow> <mat:mrow> <mat:mn>2</mat:mn> <mat:mo>?</mat:mo> </mat:mrow> </mat:msubsup> </mat:math> for high‐temperature and high‐pressure conditions is identical to that of <mat:math display="inline" altimg="urn:x-wiley:15252027:media:ggge21587:ggge21587-math-0004" wiley:location="equation/ggge21587-math-0004.png"> <mat:msubsup> <mat:mrow> <mat:mtext>SO</mat:mtext> </mat:mrow> <mat:mrow> <mat:mn>4</mat:mn> </mat:mrow> <mat:mrow> <mat:mn>2</mat:mn> <mat:mo>?</mat:mo> </mat:mrow> </mat:msubsup> </mat:math> for room temperature and atmospheric pressure. The concentrations of CO <sub>2</sub> in mid‐Okinawa Trough hydrothermal fluids determined by in situ Raman measurement are 188.4–532.3 mmol/kg, which are about 3 times higher than those obtained by traditional sampling methods (59–198 mmol/kg). However, the concentrations of <mat:math display="inline" altimg="urn:x-wiley:15252027:media:ggge21587:ggge21587-math-0005" wiley:location="equation/ggge21587-math-0005.png"> <mat:msubsup> <mat:mrow> <mat:mtext>SO</mat:mtext> </mat:mrow> <mat:mrow> <mat:mn>4</mat:mn> </mat:mrow> <mat:mrow> <mat:mn>2</mat:mn> <mat:mo>?</mat:mo> </mat:mrow> </mat:msubsup> </mat:math> calculated from in situ Raman spectra were near zero, indicating that the in situ Raman measurement avoids hydrothermal fluids contaminated with seawater. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“main”> <标题类型=“main”>抽象</ title> > 从水热通风口发出的二氧化碳作为全球碳循环的重要组成部分，可以直接影响水热生态系统。然而，传统的化学分析方法不能直接测量溶解的CO的浓度 <sub> 2 </ sub> 在高温水热流体中。尽管原位质谱已经应用于深海的测量，但它不能用于检测高温流体。在这项研究中，一种原位拉曼测量溶解CO的定量方法 <sub> 2 </ sub> 建立了适用于水热环境。 CO的拉曼相对强度 <sub> 2 </ sub> 与CO的浓度增加显示线性关系 <sub> 2 </ sub> 在调查条件下（高达300°C和40MPa），允许该方法以全球最多的方法应用于大多数水热场。此外，我们发现定量校准曲线 <mat：数学显示=“内联”Altimg =“URN：X-Wiley：15252027：GGGE21587：GGGE21587-Math-0003”Wiley：Location =“等式/ GGGE21587-Math-0003.png”> <mat：msubsup> <MAT：MROW> <mat：mtext> so </ mat：mtext> </ mat：MROW> <MAT：MROW> <MAT：MN> 4 </ MAT：MN> </ mat：MROW> <MAT：MROW> <MAT：MN> 2 </ MAT：MN> <mat：mo>？</ mat：mo> </ mat：MROW> </ mat：msubsup> </ mat：math> 对于高温和高压条件与之相同 <mat：数学显示=“内联”Altimg =“URN：X-Wiley：15252027：媒体：GGGE21587：GGGE21587-Math-0004”Wiley：Location =“等式/ GGGE21587-Math-0004.png”> <mat：msubsup> <MAT：MROW> <mat：mtext> so </ mat：mtext> </ mat：MROW> <MAT：MROW> <MAT：MN> 4 </ MAT：MN> </ mat：MROW> <MAT：MROW> <MAT：MN> 2 </ MAT：MN> <mat：mo>？</ mat：mo> </ mat：MROW> </ mat：msubsup> </ mat：math> 室温和大气压。 CO的浓度 <sub> 2 </ sub> 在原位拉曼测量确定的中冲陀瓦槽水热流体是188.4-532.3mmol / kg，比传统采样方法（59-198mmol / kg）高出3倍。但是，浓度 <mat：数学显示=“内联”Altimg =“URN：X-Wiley：15252027：媒体：GGGE21587：GGGE21587-Math-0005”Wiley：Location =“等式/ GGGE21587-Math-0005.png”> <mat：msubsup> <MAT：MROW> <mat：mtext> so </ mat：mtext> </ mat：MROW> <MAT：MROW> <MAT：MN> 4 </ MAT：MN> </ mat：MROW> <MAT：MROW> <MAT：MN> 2 </ MAT：MN> <mat：mo>？</ mat：mo> </ mat：MROW> </ mat：msubsup> </ mat：math> 根据原位拉曼光谱计算零点，表明原位拉曼测量避免了海水污染的水热流体。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23285/'>《Geochemistry, geophysics, geosystems》</a> <b style="margin: 0 2px;">|</b><span>2018年第6期</span><b style="margin: 0 2px;">|</b><span>共15页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Lianfu&option=202" target="_blank" rel="nofollow">Li Lianfu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xin&option=202" target="_blank" rel="nofollow">Zhang Xin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Luan Zhendong&option=202" target="_blank" rel="nofollow">Luan Zhendong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Zengfeng&option=202" target="_blank" rel="nofollow">Du Zengfeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xi Shichuan&option=202" target="_blank" rel="nofollow">Xi Shichuan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Bing&option=202" target="_blank" rel="nofollow">Wang Bing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Lei&option=202" target="_blank" rel="nofollow">Cao Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lian Chao&option=202" target="_blank" rel="nofollow">Lian Chao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Jun&option=202" target="_blank" rel="nofollow">Yan Jun;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> <p>CAS Key Laboratory of Marine Geology and Environment &</p> <p>Center of Deep Sea ResearchInstitute of Oceanology Chinese Academy of SciencesQingdao China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=in situ&option=203" rel="nofollow">in situ;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Raman spectroscopy&option=203" rel="nofollow">Raman spectroscopy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dissolved CO 2&option=203" rel="nofollow">dissolved CO 2;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=quantitative analysis&option=203" rel="nofollow">quantitative analysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrothermal vent fluid&option=203" rel="nofollow">hydrothermal vent fluid;</a> </p> <div class="translation"> 机译：原位;拉曼光谱;溶解CO 2;定量分析;水热通气流体; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023360459.html">In Situ Quantitative Raman Detection of Dissolved Carbon Dioxide and Sulfate in Deep‐Sea High‐Temperature Hydrothermal Vent Fluids</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Lianfu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Li 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</div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：原位定量拉曼检测溶解二氧化碳和深海高温热水通气流体中的硫酸盐</span> </p> </li> <li> <div> <b>8. </b><a class="enjiyixqcontent" href="/ntis-science-report_nasa_thesis/02071100922.html">A deep sea Hydrothermal Vent Bio-sampler for large volume in-situ filtration of hydrothermal vent fluids</a> <b>[R] </b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Behar, Alberto&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Behar, Alberto,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext= Matthews, Jaret&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> Matthews, Jaret,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext= Venkateswaran, Kasthuri&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> Venkateswaran, Kasthuri,</a> <span>2005</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：深海Hydrothermal Vent生物采样器，用于大量原位过滤热液喷口流体</span> </p> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_science_thesis/0201270289254.html">深海高温热液喷口流体原位拉曼定量探测获新突破</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=闻正&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 闻正</a> <span> <a href="/journal-cn-5187/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 科学（上海） </a> </span> <span> . 2018</span><span>,第005期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_analytical-instrumentation_thesis/0201297425190.html">原位拉曼光谱定量探测深海高温热液喷口流体获新突破</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . </a> <span> <a href="/journal-cn-8218/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 分析仪器 </a> </span> <span> . 2018</span><span>,第5期</span> </span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-journal-cn_geochimica_thesis/0201273475701.html">应用拉曼光谱定量分析流体中硫酸盐质量摩尔浓度:内标选择和流体组分对分析结果的影响</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨源显&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 杨源显</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王小林&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王小林</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=席斌斌&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,席斌斌</a> <span> <a href="/journal-cn-4899/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 地球化学 </a> </span> <span> . 2019</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-journal-cn_transactions-china-electrotechnical-society_thesis/0201230117965.html">变压器油中溶解气体拉曼剖析及定量检测优化研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈伟根&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 陈伟根</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=万福&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,万福</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=顾朝亮&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,顾朝亮</a> <span> <a href="/journal-cn-8477/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 电工技术学报 </a> </span> <span> . 2016</span><span>,第002期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_spectroscopy-spectral-analysis_thesis/0201232954999.html">以合成包裹体为腔体进行高温下流体的拉曼光谱原位分析</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈晋阳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 陈晋阳</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=郑海飞&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,郑海飞</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=曾贻善&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,曾贻善</a> <span> <a href="/journal-cn-11127/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 光谱学与光谱分析 </a> </span> <span> . 2003</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-673_thesis/020221558277.html">探测中地壳地球物理性质的新实验途径:2.观测高温高压上中地壳流体-岩石反应和对应原位测量流体性质</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张荣华&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张荣华</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张雪彤&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张雪彤</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡书敏&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,胡书敏</a> <span> <a href="/conference-cn-673/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2015年中国地球科学联合学术年会 </a> <span> <span> . 2015</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020313740571.html">深海环境及深海沉积物拉曼光谱原位定量探测技术研究--深海沉积物孔隙水及天然气水合物原位定量探测新方法</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张鑫&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张鑫</a> <span> . 2009</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120112177577.html">一种高温高压水流体环境中的原位电化学-拉曼光谱测量系统</a> <b>[P]</b> . <span> 中国专利： CN112179968A </span> <span> . 2021-01-05</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120213813552.html">高温高压水流体环境中的原位电化学-拉曼光谱测量系统</a> <b>[P]</b> . <span> 中国专利： CN213875522U </span> <span> . 2021-08-03</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130418562064.html">Hydrothermal energy and deep sea resource recovery system, hydrothermal fluid delivery system, and method for recovering resources contained in hydrothermal fluid</a> <b>[P]</b> . <span> 外国专利： <!-- 日本专利： --> JP5395072B2 </span> <span> . 2014-01-22</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：热能和深海资源回收系统，热液输送系统以及热液中所含资源的回收方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130450934930.html">METHOD FOR DISSOLVING LOW-PURITY GASEOUS CARBON DIOXIDE INTO SEAWATER AND FEEDING THE GAS INTO DEEP SEA AND APPARATUS THEREFOR</a> <b>[P]</b> . <span> 外国专利： <!-- 日本专利： --> JP2000070702A </span> <span> . 2000-03-07</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：将低纯度气态二氧化碳溶解在海水中并将气体注入深海及其装置的方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130452832653.html">Method and apparatus for dissolving low-purity carbon dioxide gas in seawater and sending it to the deep sea</a> <b>[P]</b> . <span> 外国专利： <!-- 日本专利： --> JP2958460B1 </span> <span> . 1999-10-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：将低纯度二氧化碳气体溶解在海水中并将其输送到深海的方法和设备 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704023360459','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="" 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