(S)-Selective Dynamic Kinetic Resolution of Allylic Alcohols by Enzyme-Metal Bicatalysis

Mahn-Joo Kim; Han Ki Lee; Jaiwook Park

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(S)-Selective Dynamic Kinetic Resolution of Allylic Alcohols by Enzyme-Metal Bicatalysis

机译：酶金属双催化的烯丙醇的（S）-选择性动态动力学拆分

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摘要

Dynamic kinetic resolution (DKR) provides a useful methodology for the conversion of racemic substrates to single enantiomeric products.In the last decade,a new approach for DKR has been intensively explored,in which an enzyme as the resolution catalyst is combined with a metal or metal complex as the racemization catalyst.

机译：动态动力学拆分（DKR）为外消旋底物向单一对映体产物的转化提供了有用的方法。在过去的十年中，DKR的新方法得到了广泛的研究，其中酶作为拆分催化剂与金属或金属结合使用。金属配合物作为外消旋催化剂。

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《Bulletin of the Korean Chemical Society》 |2007年第11期|共3页
作者
Mahn-Joo Kim; Han Ki Lee; Jaiwook Park;
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正文语种 eng
中图分类化学工业;
关键词
Dynamic kinetic resolution; Allylic alcohol; Subtilisin; Ruthenium; Enzyme-metal combination;

机译：动态动力学拆分烯丙醇枯草杆菌蛋白酶钌酶金属结合;

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专利

1. (S)-Selective Dynamic Kinetic Resolution of Allylic Alcohols by Enzyme-Metal Bicatalysis [J] . Mahn-Joo Kim, Han Ki Lee, Jaiwook Park Bulletin of the Korean Chemical Society . 2007,第11期

机译：酶金属双催化的烯丙醇的（S）-选择性动态动力学拆分
2. Highly Selective Palladium Catalyzed Kinetic Resolution and Enantioselective Substitution of Racemic Allylic Carbonates with Sulfur Nucleophiles: Asymmetric Synthesis of Allylic Sulfides, Allylic Sulfones, and Allylic Alcohols [J] . Hans-Joachim Gais, Thomas Jagusch, Nicole Spalthoff, Chemistry: A European journal . 2003,第17期

机译：高选择性钯催化硫代亲核试剂的消旋烯丙基碳酸酯的动力学拆分和对映选择性取代：烯丙基硫化物，烯丙基砜和烯丙醇的不对称合成
3. Dynamic kinetic resolution of secondary alcohols by enzyme-metal combinations in ionic liquid [J] . Kim MJ, Kim HM, Kim D, Green chemistry . 2004,第9期

机译：离子液体中酶金属结合对仲醇的动力学动力学拆分
4. Phase-Transfer Catalytic Dynamic Kinetic Resolution of AminoAcid Esters with Water and Alcohols as Nucleophiles [C] . Kodai Wakafuji, Kaoru Kobayashi, Hyemin Cho 日本化学会春季年会 . 2020

机译：用水和醇作为亲核试剂的氨基酸酯的相转移催化动力学分辨率
5. Investigation of the Addition of a Kinetic Bimolecular Fragment Coupling Step to the Re2O7-Catalyzed Transposition and Cyclization of Allylic Alcohols and Examination of the Effects of Acetonitrile [D] . Anderson, Shelby Marie. 2020

机译：对烯丙基醇的RE2O7催化转子添加动力学分散片段偶联步骤的研究及乙腈的影响检查
6. Kinetic resolution of racemic allylic alcohols via iridium-catalyzed asymmetric hydrogenation: scope synthetic applications and insight into the origin of selectivity [O] . Haibo Wu, Cristiana Margarita, Jira Jongcharoenkamol, 2021

机译：通过铱催化的不对称氢化的外消旋烯丙基醇的动力学分辨率：范围合成应用和对选择性起源的洞察
7. Migratory Dynamic Kinetic Resolution of Carbocyclic Allylic Alcohols [O] . Sapu, Chicco Manzuna, Görbe, Tamás, Lihammar, Richard, 2014

机译：碳环烯丙基醇的迁移动力学动力学拆分

(S)-Selective Dynamic Kinetic Resolution of Allylic Alcohols by Enzyme-Metal Bicatalysis

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