Palladium-Catalyzed N-Arylation of Amines and Amides with Aryltrimethylgermanes

Zhang Qiang; Liu Cunfang; Shi Juan; Xu Qiong; Jin Lingxia; Zhao Chaibin; Zhang Tianlei

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Palladium-Catalyzed N-Arylation of Amines and Amides with Aryltrimethylgermanes

机译：钯催化的胺基和酰胺基与芳基三甲基锗烷的N-芳基化

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摘要

Described herein is a novel palladium-catalyzed C-N bond-formation reaction employing aryltrimethylgermanes as the new arylating reagents. Primary/secondary amines or even amides could be smoothly arylated to provide the corresponding N-arylation products in moderate to excellent yields.

机译：本文描述了使用芳基三甲基锗烷作为新的芳基化试剂的新颖的钯催化的C-N键形成反应。伯/仲胺或什至酰胺可以平滑地芳基化，以中等到极好的收率提供相应的N-芳基化产物。

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《Synlett》 |2016年第13期|共4页
作者
Zhang Qiang; Liu Cunfang; Shi Juan; Xu Qiong; Jin Lingxia; Zhao Chaibin; Zhang Tianlei;
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正文语种 eng
中图分类有机化学理论、物理有机化学;
关键词
N-arylation; amine; amide; aryltrimethylgermane;

机译：N-芳基化;胺;酰胺;芳基三甲基锗烷;

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专利

1. Palladium-Catalyzed N-Arylation of Amines and Amides with Aryltrimethylgermanes [J] . Zhang Qiang, Liu Cunfang, Shi Juan, Synlett . 2016,第13期

机译：钯催化的胺基和酰胺基与芳基三甲基锗烷的N-芳基化
2. Heterogeneous Cu~(II)-Catalysed Solvent-Controlled Selective N-Arylation of Cyclic Amides and Amines with Bromo-iodoarenes [J] . Debasish Kundu, Sukalyan Bhadra, Nirmalya Mukherjee, Chemistry: A European journal . 2013,第46期

机译：异质铜〜（II）催化的环酰胺和胺与溴碘芳烃的溶剂控制的选择性N-芳基化
3. Heterogeneous Cu~(II)-Catalysed Solvent-Controlled Selective N-Arylation of Cyclic Amides and Amines with Bromo-iodoarenes [J] . Debasish Kundu, Sukalyan Bhadra, Nirmalya Mukherjee, Chemistry: A European journal . 2013,第46期

机译：异质铜〜（II）催化的环酰胺和胺与溴碘芳烃的溶剂控制的选择性N-芳基化
4. Synthesis of Carbazole Derivatives by Palladium Catalyzed Double N-Arylation of Amines [C] . Yuko Hidehira, Koji Nakano, Atsushi Kuwahara, Symposium on Organometallic Chemistry . 2004

机译：钯催化酶衍生物的合成衍生物的双N-芳基芳基
5. Palladium-catalyzed alkoxycarbonylation and aminocarbonylation of terminal alkynes: Synthesis and applications of alpha,beta-unsaturated esters and amides. Computational study of the reaction mechanism. [D] . Suleiman, Rami. 2010

机译：钯催化末端炔烃的烷氧基羰基化和氨基羰基化：α，β-不饱和酯和酰胺的合成和应用。反应机理的计算研究。
6. N-Arylation of amines amides imides and sulfonamides with arylboroxines catalyzed by simple copper salt/EtOH system [O] . Zhang-Guo Zheng, Jun Wen, Na Wang, 2008

机译：简单铜盐/ EtOH体系催化的胺酰胺酰亚胺和磺酰胺与芳基硼氧烷的N-芳基化
7. N-Arylation of amines, amides, imides and sulfonamides with arylboroxines catalyzed by simple copper salt/EtOH system [O] . Zheng, Zhang-Guo, Wen, Jun, Wang, Na, 2008

机译：简单铜盐/ EtOH体系催化的胺，酰胺，酰亚胺和磺酰胺与芳基硼氧烷的N-芳基化

Palladium-Catalyzed N-Arylation of Amines and Amides with Aryltrimethylgermanes

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