Lewis acid-promoted synthesis of unsymmetrical and highly functionalized carbazoles and dibenzofurans from biaryl triazenes: Application for the total synthesis of clausine C, clausine R, and clauraila A

Yang W.; Zhou J.; Wang B.; Ren H.

首页> 外文期刊>Chemistry: A European journal >Lewis acid-promoted synthesis of unsymmetrical and highly functionalized carbazoles and dibenzofurans from biaryl triazenes: Application for the total synthesis of clausine C, clausine R, and clauraila A

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Lewis acid-promoted synthesis of unsymmetrical and highly functionalized carbazoles and dibenzofurans from biaryl triazenes: Application for the total synthesis of clausine C, clausine R, and clauraila A

机译：路易斯酸促进的由联芳基三氮烯合成不对称和高度官能化的咔唑和二苯并呋喃：用于总合成clausine C，clausine R和clauraila A

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A natural approach: A Lewis acid-promoted nucleophilic aromatic substitution approach to the regioselective synthesis of highly substituted carbazoles and dibenzofurans has been developed. The annulation process is applied to the total synthesis of carbazole alkaloids clausine C, clausine R, and clauraila A (see scheme).

机译：一种自然方法：已开发出路易斯酸促进的亲核芳香族取代方法，用于高度取代的咔唑和二苯并呋喃的区域选择性合成。环化工艺应用于咔唑生物碱克劳斯汀C，克劳斯汀R和克劳拉艾拉A的全合成（请参阅方案）。

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《Chemistry: A European journal》 |2011年第49期|共5页
作者
Yang W.; Zhou J.; Wang B.; Ren H.;
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正文语种 eng
中图分类应用化学;
关键词
alkaloids; carbazole; dibenzofuran; nucleophilic substitution; regioselectivity; triazene;

机译：生物碱;咔唑;二苯并呋喃;亲核取代;区域选择性;三氮烯;

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1. Lewis acid-promoted synthesis of unsymmetrical and highly functionalized carbazoles and dibenzofurans from biaryl triazenes: Application for the total synthesis of clausine C, clausine R, and clauraila A [J] . Yang W., Zhou J., Wang B., Chemistry: A European journal . 2011,第49期

机译：路易斯酸促进的由联芳基三氮烯合成不对称和高度官能化的咔唑和二苯并呋喃：用于总合成clausine C，clausine R和clauraila A
2. Transition metals in organic synthesis, part 85. A general approach to 1,6-dioxygenated carbazole alkaloids - First total synthesis of clausine G, clausine I, and clausine Z [J] . Borger C, Knolker HJ Synlett . 2008,第11期

机译：有机合成中的过渡金属，第85部分。1,6-二加氧咔唑生物碱的一般方法-克劳辛G，克劳辛I和克劳辛Z的首次全合成
3. First total synthesis of the 7-oxygenated carbazole alkaloids clauszoline-K,3-formyl-7-hydroxycarbazole,clausine M,clausine N and the anti-HIV active siamenol using a highly efficient palladium-catalyzed approach [J] . Micha P.Krahl, Anne Jager, Tilo Krause Organic & biomolecular chemistry . 2006,第17期

机译：使用高效钯催化方法首次全合成7-氧化咔唑生物碱clauszoline-K，3-formyl-7-hydroxycarbazole，clausine M，clausine N和抗HIV活性的siamenol
4. Synthesis and characterization of unsymmetrically branched alkyl chains carbazole-based polymer [C] . Mohd Sani Sarjadi, Shu Er Tan, Xin Lin Wong, Joint Conference on Chemistry . 2020

机译：非对称支链烷基链咔唑基聚合物的合成与表征
5. An application of the intramolecular Heck reaction: A new strategy in the synthesis of Hasubanan alkaloids. Preparation of unsymmetrical biaryls via the Stille cross-coupling reaction: Synthesis of highly functional intermediates towards the synthesis of vindoline. [D] . Frank, Anthony Joseph. 2002

机译：分子内Heck反应的应用：合成Hasubanan生物碱的新策略。通过Stille交叉偶联反应制备不对称的联芳基：合成高功能性中间体，合成长春新碱。
6. Lewis acid-promoted cascade reaction for the synthesis of Michael acceptors and its application in a dimerization reaction [O] . Xiao-Jing Zhao, Jie Zhao, Xin Sun, -1

机译：路易斯酸促进的级联反应用于迈克尔受体的合成及其在二聚反应中的应用
7. Supported palladium hydroxide-catalyzed intramolecular double C H bond functionalization for synthesis of carbazoles and dibenzofurans [O] . Tamao Ishida, Ryosuke Tsunoda, Zhenzhong Zhang, 2014

机译：支持钯氢氧化钯催化的分子内双C H键官能化，用于合成咔唑和二苯并呋喃

Lewis acid-promoted synthesis of unsymmetrical and highly functionalized carbazoles and dibenzofurans from biaryl triazenes: Application for the total synthesis of clausine C, clausine R, and clauraila A

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